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Molecular water oxidation catalysis : a key topic for new sustainable energy conversion schemes / / Antoni Llobet, editor
Molecular water oxidation catalysis : a key topic for new sustainable energy conversion schemes / / Antoni Llobet, editor
Pubbl/distr/stampa West Sussex, England : , : John Wiley & Sons, , 2014
Descrizione fisica 1 online resource (305 p.)
Disciplina 621.31/242
Soggetto topico Energy harvesting
Water - Purification - Oxidation - By-products
Renewable energy sources
Electric power production from chemical action
ISBN 1-118-69862-2
1-118-69863-0
1-118-69864-9
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto Cover; Title Page; Copyright; Contents; List of Contributors; Preface; Chapter 1 Structural Studies of Oxomanganese Complexes for Water Oxidation Catalysis; 1.1 Introduction; 1.2 Structural Studies of the OEC; 1.3 The Dark-Stable State of the OEC; 1.4 Biomimetic Oxomanganese Complexes; 1.5 Base-Assisted O-O Bond Formation; 1.6 Biomimetic Mn Catalysts for Artificial Photosynthesis; 1.7 Conclusion; Acknowledgments; References; Chapter 2 O-O Bond Formation by a Heme Protein: The Unexpected Efficiency of Chlorite Dismutase; 2.1 Introduction; 2.2 Origins of O2-Evolving Chlorite Dismutases (Clds)
2.3 Major Structural Features of the Proteins and their Active Sites2.4 Efficiency, Specificity, and Stability; 2.5 Mechanistic Insights from Surrogate Reactions with Peracids and Peroxide; 2.6 Possible Mechanisms; 2.7 Conclusion; Acknowledgements; References; Chapter 3 Ru-Based Water Oxidation Catalysts; 3.1 Introduction; 3.2 Proton-Coupled Electron Transfer (PCET) and Water Oxidation Thermodynamics; 3.3 O-O Bond Formation Mechanisms; 3.4 Polynuclear Ru Water Oxidation Catalysts; 3.5 Mononuclear Ru WOCs; 3.6 Anchored Molecular Ru WOCs; 3.7 Light-Induced Ru WOCs; 3.8 Conclusion
AcknowledgmentsReferences; Chapter 4 Towards the Visible Light-Driven Water Splitting Device: Ruthenium Water Oxidation Catalysts with Carboxylate-Containing Ligands; 4.1 Introduction; 4.2 Binuclear Ru Complexes; 4.3 Mononuclear Ru Complexes; 4.3.1 Ru-O2N-N3 Analogs; 4.3.2 Ru-O2N2-N2 Analogs; 4.4 Homogeneous Light-Driven Water Oxidation; 4.4.1 The Three-Component System; 4.4.2 The Supramolecular Assembly Approach; 4.5 Water Oxidation Device; 4.5.1 Electrochemical Water Oxidation Anode; 4.5.2 Photo-Anode for Water Oxidation; 4.6 Conclusion; References
Chapter 5 Water Oxidation by Ruthenium Catalysts with Non-Innocent Ligands5.1 Introduction; 5.2 Water Oxidation Catalyzed by Dinuclear Ruthenium Complexes with NILs; 5.3 Water Oxidation by Intramolecular O-O Coupling with [Ru II2(μ-Cl)(bpy)2(btpyan)]3+; 5.4 Mononuclear Ru-Aqua Complexes with a Dioxolene Ligand; 5.4.1 Structural Characterization; 5.4.2 Theoretical and Electrochemical Characterization; 5.5 Mechanistic Investigation of Water Oxidation by Dinuclear Ru Complexes with NILs: Characterization of Key Intermediates; References
Chapter 6 Recent Advances in the Field of Iridium-Catalyzed Molecular Water Oxidation6.1 Introduction; 6.2 Bernhard 2008 [11]; 6.3 Crabtree 2009 [12]; 6.4 Crabtree 2010 [13]; 6.5 Macchioni 2010 [14]; 6.6 Albrecht/Bernhard 2010 [15]; 6.7 Hetterscheid/Reek 2011 [16,17]; 6.8 Crabtree 2011 [18]; 6.9 Crabtree 2011 [19]; 6.10 Lin 2011 [20]; 6.11 Macchioni 2011 [21]; 6.12 Grotjahn 2011 [22]; 6.13 Fukuzumi 2011 [23]; 6.14 Lin 2012 [24]; 6.15 Crabtree 2012 [25-27]; 6.16 Albrecht/Bernhard 2012 [28]; 6.17 Crabtree 2012 [29]; 6.18 Beller 2012 [30]; 6.19 Lin 2012 [31]; 6.20 Lloblet and Macchioni 2012 [33]
6.21 Analysis
Record Nr. UNINA-9910139112103321
West Sussex, England : , : John Wiley & Sons, , 2014
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui
Molecular water oxidation catalysis : a key topic for new sustainable energy conversion schemes / / Antoni Llobet, editor
Molecular water oxidation catalysis : a key topic for new sustainable energy conversion schemes / / Antoni Llobet, editor
Pubbl/distr/stampa West Sussex, England : , : John Wiley & Sons, , 2014
Descrizione fisica 1 online resource (305 p.)
Disciplina 621.31/242
Soggetto topico Energy harvesting
Water - Purification - Oxidation - By-products
Renewable energy sources
Electric power production from chemical action
ISBN 1-118-69862-2
1-118-69863-0
1-118-69864-9
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto Cover; Title Page; Copyright; Contents; List of Contributors; Preface; Chapter 1 Structural Studies of Oxomanganese Complexes for Water Oxidation Catalysis; 1.1 Introduction; 1.2 Structural Studies of the OEC; 1.3 The Dark-Stable State of the OEC; 1.4 Biomimetic Oxomanganese Complexes; 1.5 Base-Assisted O-O Bond Formation; 1.6 Biomimetic Mn Catalysts for Artificial Photosynthesis; 1.7 Conclusion; Acknowledgments; References; Chapter 2 O-O Bond Formation by a Heme Protein: The Unexpected Efficiency of Chlorite Dismutase; 2.1 Introduction; 2.2 Origins of O2-Evolving Chlorite Dismutases (Clds)
2.3 Major Structural Features of the Proteins and their Active Sites2.4 Efficiency, Specificity, and Stability; 2.5 Mechanistic Insights from Surrogate Reactions with Peracids and Peroxide; 2.6 Possible Mechanisms; 2.7 Conclusion; Acknowledgements; References; Chapter 3 Ru-Based Water Oxidation Catalysts; 3.1 Introduction; 3.2 Proton-Coupled Electron Transfer (PCET) and Water Oxidation Thermodynamics; 3.3 O-O Bond Formation Mechanisms; 3.4 Polynuclear Ru Water Oxidation Catalysts; 3.5 Mononuclear Ru WOCs; 3.6 Anchored Molecular Ru WOCs; 3.7 Light-Induced Ru WOCs; 3.8 Conclusion
AcknowledgmentsReferences; Chapter 4 Towards the Visible Light-Driven Water Splitting Device: Ruthenium Water Oxidation Catalysts with Carboxylate-Containing Ligands; 4.1 Introduction; 4.2 Binuclear Ru Complexes; 4.3 Mononuclear Ru Complexes; 4.3.1 Ru-O2N-N3 Analogs; 4.3.2 Ru-O2N2-N2 Analogs; 4.4 Homogeneous Light-Driven Water Oxidation; 4.4.1 The Three-Component System; 4.4.2 The Supramolecular Assembly Approach; 4.5 Water Oxidation Device; 4.5.1 Electrochemical Water Oxidation Anode; 4.5.2 Photo-Anode for Water Oxidation; 4.6 Conclusion; References
Chapter 5 Water Oxidation by Ruthenium Catalysts with Non-Innocent Ligands5.1 Introduction; 5.2 Water Oxidation Catalyzed by Dinuclear Ruthenium Complexes with NILs; 5.3 Water Oxidation by Intramolecular O-O Coupling with [Ru II2(μ-Cl)(bpy)2(btpyan)]3+; 5.4 Mononuclear Ru-Aqua Complexes with a Dioxolene Ligand; 5.4.1 Structural Characterization; 5.4.2 Theoretical and Electrochemical Characterization; 5.5 Mechanistic Investigation of Water Oxidation by Dinuclear Ru Complexes with NILs: Characterization of Key Intermediates; References
Chapter 6 Recent Advances in the Field of Iridium-Catalyzed Molecular Water Oxidation6.1 Introduction; 6.2 Bernhard 2008 [11]; 6.3 Crabtree 2009 [12]; 6.4 Crabtree 2010 [13]; 6.5 Macchioni 2010 [14]; 6.6 Albrecht/Bernhard 2010 [15]; 6.7 Hetterscheid/Reek 2011 [16,17]; 6.8 Crabtree 2011 [18]; 6.9 Crabtree 2011 [19]; 6.10 Lin 2011 [20]; 6.11 Macchioni 2011 [21]; 6.12 Grotjahn 2011 [22]; 6.13 Fukuzumi 2011 [23]; 6.14 Lin 2012 [24]; 6.15 Crabtree 2012 [25-27]; 6.16 Albrecht/Bernhard 2012 [28]; 6.17 Crabtree 2012 [29]; 6.18 Beller 2012 [30]; 6.19 Lin 2012 [31]; 6.20 Lloblet and Macchioni 2012 [33]
6.21 Analysis
Record Nr. UNINA-9910822661103321
West Sussex, England : , : John Wiley & Sons, , 2014
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui