Asymmetric synthesis in organophosphorus chemistry : synthetic methods, catalysis, and applications / / Oleg I. Kolodiazhnyi |
Autore | Kolodiazhnyi Oleg I. |
Pubbl/distr/stampa | Weinheim, Germany : , : Wiley-VCH, , 2017 |
Descrizione fisica | 1 online resource (393 p.) |
Disciplina | 547.07 |
Soggetto topico |
Organophosphorus compounds
Asymmetric synthesis |
ISBN |
3-527-34153-6
3-527-34151-X 3-527-34154-4 |
Formato | Materiale a stampa ![]() |
Livello bibliografico | Monografia |
Lingua di pubblicazione | eng |
Nota di contenuto |
Cover; Title Page; Copyright; Dedication; Contents; Preface; Abbreviations; Chapter 1 Fundamentals of the Stereochemistry of Organophosphorus Compounds; 1.1 Historical Background; 1.2 Some Common Definitions in Stereochemistry; 1.3 Determination of Enantiomer Composition; 1.3.1 Method of Nuclear Magnetic Resonance; 1.3.1.1 Chiral Solvating Agents; 1.3.1.2 Complexes of Metals (Shift Reagents); 1.3.1.3 Chiral Derivatizing Agents for NMR; 1.3.2 Chromatographic Methods of Analysis; 1.3.2.1 Gas Chromatography; 1.3.2.2 Liquid Chromatography; 1.4 Determination of the Absolute Configuration
1.4.1 X-ray Crystal Analysis1.4.2 Method of Chemical Correlation; 1.4.3 The Assignment of Absolute Configuration by NMR; 1.5 Asymmetric Induction and Stereochemistry; 1.5.1 Asymmetric Induction; 1.5.2 Asymmetric Synthesis; 1.5.3 Asymmetric Transformation; 1.5.4 An Enantioselective Reaction; 1.5.5 Enantioselective Synthesis; 1.6 Summary; References; Chapter 2 Asymmetric Synthesis of P-Chirogenic Phosphorus Compounds; 2.1 Introduction; 2.2 Low-Coordinated Phosphorus Compounds; 2.3 Trivalent Tricoordinated Phosphorus Compounds; 2.3.1 Configuration Stability of P(III)-Compounds 2.3.2 Asymmetric Nucleophilic Substitution at P (III)2.3.2.1 Secondary Alcohols as Chiral Auxiliaries; 2.3.2.2 Optically Active Amines as Chiral Auxiliaries; 2.3.2.3 Ephedrine as Inductor of Chirality at P(III); 2.3.3 Asymmetric Oxidation of P(III) Compounds; 2.3.4 Asymmetric Electrophilic Substitution at P(III); 2.3.4.1 Asymmetric Michaelis-Arbuzov Reaction; 2.4 Pentavalent P(IV)-Phosphorus Compounds; 2.4.1 Introduction; 2.4.2 Nucleophilic Substitution Reactions; 2.4.2.1 Nucleophilic Substitution at P(IV) with Chiral Alcohol; 2.4.2.2 Nucleophilic Substitution at P(IV) with Chiral Amines 2.5 Chiral P(V) and P(VI) Phosphorus Compounds2.6 Summary; References; Chapter 3 Phosphorus Compounds with Chiral Side-Chain Centers; 3.1 Introduction; 3.2 Asymmetric Induction in Side Chains; 3.2.1 Transfer of Chirality from Phosphorus to Other Centers; 3.2.1.1 Chiral Phosphorus-Stabilized Anions; 3.2.1.2 1,2-Asymmetric Induction; 3.2.1.3 1,4-Asymmetric Induction; 3.3 Enantioselective Olefination; 3.4 Stereoselective Addition of Phosphorous Nucleophiles to C=X Bonds; 3.4.1 Phospha-Aldol Reaction; 3.4.2 Phospha-Mannich Reaction; 3.4.3 Phospha-Michael Reaction; 3.5 Asymmetric Reduction 3.6 Asymmetric Oxidation3.7 C-Modification; 3.8 Asymmetric Cycloaddition; 3.9 Multiple Stereoselectivity; 3.10 Summary; References; Chapter 4 Asymmetric Catalysis with Metal Complexes; 4.1 Introduction; 4.2 Asymmetric Catalytic Hydrogenation and Other Reactions of Reduction; 4.2.1 Hydrogenation of C=C Phosphorus Compounds; 4.2.2 Hydrogenation of C=O Phosphorus Compounds; 4.3 Asymmetric Reduction and Oxidation; 4.3.1 Reduction of C=O, C=N, and C=C bonds; 4.3.2 Asymmetric Oxidation; 4.4 Electrophilic Asymmetric Catalysis; 4.4.1 Catalytic Electrophilic Substitution at the Phosphorus Atom 4.4.1.1 Alkylation and Arylation of P(III) Compounds |
Record Nr. | UNINA-9910134858903321 |
Kolodiazhnyi Oleg I.
![]() |
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Weinheim, Germany : , : Wiley-VCH, , 2017 | ||
![]() | ||
Lo trovi qui: Univ. Federico II | ||
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Asymmetric synthesis in organophosphorus chemistry : synthetic methods, catalysis, and applications / / Oleg I. Kolodiazhnyi |
Autore | Kolodiazhnyi Oleg I. |
Pubbl/distr/stampa | Weinheim, Germany : , : Wiley-VCH, , 2017 |
Descrizione fisica | 1 online resource (393 p.) |
Disciplina | 547.07 |
Soggetto topico |
Organophosphorus compounds
Asymmetric synthesis |
ISBN |
3-527-34153-6
3-527-34151-X 3-527-34154-4 |
Formato | Materiale a stampa ![]() |
Livello bibliografico | Monografia |
Lingua di pubblicazione | eng |
Nota di contenuto |
Cover; Title Page; Copyright; Dedication; Contents; Preface; Abbreviations; Chapter 1 Fundamentals of the Stereochemistry of Organophosphorus Compounds; 1.1 Historical Background; 1.2 Some Common Definitions in Stereochemistry; 1.3 Determination of Enantiomer Composition; 1.3.1 Method of Nuclear Magnetic Resonance; 1.3.1.1 Chiral Solvating Agents; 1.3.1.2 Complexes of Metals (Shift Reagents); 1.3.1.3 Chiral Derivatizing Agents for NMR; 1.3.2 Chromatographic Methods of Analysis; 1.3.2.1 Gas Chromatography; 1.3.2.2 Liquid Chromatography; 1.4 Determination of the Absolute Configuration
1.4.1 X-ray Crystal Analysis1.4.2 Method of Chemical Correlation; 1.4.3 The Assignment of Absolute Configuration by NMR; 1.5 Asymmetric Induction and Stereochemistry; 1.5.1 Asymmetric Induction; 1.5.2 Asymmetric Synthesis; 1.5.3 Asymmetric Transformation; 1.5.4 An Enantioselective Reaction; 1.5.5 Enantioselective Synthesis; 1.6 Summary; References; Chapter 2 Asymmetric Synthesis of P-Chirogenic Phosphorus Compounds; 2.1 Introduction; 2.2 Low-Coordinated Phosphorus Compounds; 2.3 Trivalent Tricoordinated Phosphorus Compounds; 2.3.1 Configuration Stability of P(III)-Compounds 2.3.2 Asymmetric Nucleophilic Substitution at P (III)2.3.2.1 Secondary Alcohols as Chiral Auxiliaries; 2.3.2.2 Optically Active Amines as Chiral Auxiliaries; 2.3.2.3 Ephedrine as Inductor of Chirality at P(III); 2.3.3 Asymmetric Oxidation of P(III) Compounds; 2.3.4 Asymmetric Electrophilic Substitution at P(III); 2.3.4.1 Asymmetric Michaelis-Arbuzov Reaction; 2.4 Pentavalent P(IV)-Phosphorus Compounds; 2.4.1 Introduction; 2.4.2 Nucleophilic Substitution Reactions; 2.4.2.1 Nucleophilic Substitution at P(IV) with Chiral Alcohol; 2.4.2.2 Nucleophilic Substitution at P(IV) with Chiral Amines 2.5 Chiral P(V) and P(VI) Phosphorus Compounds2.6 Summary; References; Chapter 3 Phosphorus Compounds with Chiral Side-Chain Centers; 3.1 Introduction; 3.2 Asymmetric Induction in Side Chains; 3.2.1 Transfer of Chirality from Phosphorus to Other Centers; 3.2.1.1 Chiral Phosphorus-Stabilized Anions; 3.2.1.2 1,2-Asymmetric Induction; 3.2.1.3 1,4-Asymmetric Induction; 3.3 Enantioselective Olefination; 3.4 Stereoselective Addition of Phosphorous Nucleophiles to C=X Bonds; 3.4.1 Phospha-Aldol Reaction; 3.4.2 Phospha-Mannich Reaction; 3.4.3 Phospha-Michael Reaction; 3.5 Asymmetric Reduction 3.6 Asymmetric Oxidation3.7 C-Modification; 3.8 Asymmetric Cycloaddition; 3.9 Multiple Stereoselectivity; 3.10 Summary; References; Chapter 4 Asymmetric Catalysis with Metal Complexes; 4.1 Introduction; 4.2 Asymmetric Catalytic Hydrogenation and Other Reactions of Reduction; 4.2.1 Hydrogenation of C=C Phosphorus Compounds; 4.2.2 Hydrogenation of C=O Phosphorus Compounds; 4.3 Asymmetric Reduction and Oxidation; 4.3.1 Reduction of C=O, C=N, and C=C bonds; 4.3.2 Asymmetric Oxidation; 4.4 Electrophilic Asymmetric Catalysis; 4.4.1 Catalytic Electrophilic Substitution at the Phosphorus Atom 4.4.1.1 Alkylation and Arylation of P(III) Compounds |
Record Nr. | UNINA-9910814764703321 |
Kolodiazhnyi Oleg I.
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Weinheim, Germany : , : Wiley-VCH, , 2017 | ||
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Lo trovi qui: Univ. Federico II | ||
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Phosphorus ylides : chemistry and application in organic synthesis / / Oleg I. Kolodiazhnyi |
Autore | Kolodiazhnyi Oleg I. |
Pubbl/distr/stampa | Weinheim, [Germany] : , : Wiley-VCH, , 1999 |
Descrizione fisica | 1 online resource (569 p.) |
Disciplina |
547.05
547.07 547.070459 |
Soggetto topico |
Ylides
Organophosphorus compounds Organophosphorus compounds - Synthesis |
Soggetto genere / forma | Electronic books. |
ISBN |
1-281-84249-4
9786611842499 3-527-61390-0 3-527-61391-9 |
Formato | Materiale a stampa ![]() |
Livello bibliografico | Monografia |
Lingua di pubblicazione | eng |
Nota di contenuto |
Phosphorus Ylides; Contents; 1 Introduction; 1.1 Historiography; 1.2 Types of Phosphorus Ylides and Structure of Book; 1.3 Nornenclature; References; 2 C,P-Carbo-Substituted Phosphorus Ylides; 2.1 Introduction; 2.1.1 Types of C,P-Carbo-Substituted Posphorus Ylides; 2.2 Preparation; 2.2.1 Synthesis from Phosphonium Salts; 2.2.1.1 Dehydrohalogenation of Phosphonium Salts; 2.2.1.2 Synthesis from a-Silyl and a-Stannyl-Substituted Phosphonium Salts; 2.2.1.3 Preparation in Heterogeneous Media; 2.2.1.4 Electrochemical Method; 2.2.1.5 Ultrasound; 2.2.2 Modification of Simple Phosphorus Ylides
2.2.2.1 Acylation2.2.2.2 Alkylation; 2.2.2.3 Arylation; 2.2.3 Addition of Tertiary Phosphines to Compounds Containing Multiple Bonds; 2.2.3.1 Alkenes; 2.2.3.2 Alkynes; 2.2.4 Reaction of Tetracoordinatc Phosphorus Compounds with Multiple-Bonded Compounds; 2.2.5 Modification of the Side-Chain; 2.2.6 Miscellaneous Methods; 2.2.6.1 Formation from Carbenes; 2.2.6.2 Phosphorylation of Cornpounds with an Active Methylene Group; 2.3 Chemical Properties; 2.3.1 Stability; 2.3.2 Transformations Accompanied by Cleavage of the P=C Bond; 2.3.2.1 Thermolysis; 2.3.2.2 Photolysis 2.3.2.3 Oxidation-Industrial Synthesis of B-Carotene2.3.2.4 Reactions with Elemental Sulfur and Selenium; 2.3.2.5 Reduction; 2.3.3.6 Hydrolysis of Ylides; 2.3.2.7 Applications in Organic Synthesis; 2.3.3 Substitution at the Ylidic Carbon Atom; 2.3.3.1 Reactions with Alkylation Reagents; 2.3.3.2 Reactions with Acylation Reagents; 2.3.3.3 Examples in Natural Compound Synthesis; 2.3.4 Reactions with Compounds Containing Multiple Bonds; 2.3.4.1 Compounds Containing Carbon-Carbon Multiple Bonds; 2.3.4.2 Reactions with Compounds Containing Carbon-Heteroatom or Heteroatom-Heteroatom Multiple Bonds 2.3.5 Reactions with 1,3-Dipolar Compounds. Synthesis of Heterocyclic Systems2.3.5.1 Reaction with Aziridines and Azomethine Ylides-Synthesis of Pyrrolines; 2.3.5.2 Oxides of Azomethines; 2.3.5.3 Azides-Synthesis of 1,2, 3-Triazoles; 2.3.5.4 Reaction with Nitrile Oxides. Nitrilimines and Nitrilylides - Synthesis of Pyrazoles and Isoxazoles; References; 3 Cumulene Ylides; 3.1 Introduction; 3.1.1 The Structure of Phosphacumulene Ylides; 3.2 Phosphaketene Ylides; 3.2.1 Chemical Properties; 3.2.2 Dimerization; 3.2.3 Addition of Compounds Bearing a Mobile Hydrogen Atom 3.2.4 [2+2] Cycloaddition Reactions3.2.5 1,3-Dipolar Addition Reactions; 3.2.6 [4+2]-Cycloaddition Reactions; 3.2.7 Miscellaneous Reactions; 3.3 Phosphaketeneacetal Ylides; 3.4 Phosphaallene Ylides and Phosphacumulene Ylides; 3.5 Application in Natural Product Synthesis; 3.6 Carbodiphophoranes; 3.6.1 Structural Studies of Carbodiphosphoranes; References; 4 C-Heterosubstituted Phosphorus Ylides; 4.1 Introduction; 4.2 Phosphorus Ylides Substituted on the a-Carbon by Atoms of Element Groups I-IV; 4.2.1 Ylides Containing Group 1A and IIA Elements; 4.2.2 Ylides Containing Group IIIA Elements 4.2.3 Ylides Containing Group IVA Elements |
Record Nr. | UNINA-9910144281903321 |
Kolodiazhnyi Oleg I.
![]() |
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Weinheim, [Germany] : , : Wiley-VCH, , 1999 | ||
![]() | ||
Lo trovi qui: Univ. Federico II | ||
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Phosphorus ylides : chemistry and application in organic synthesis / / Oleg I. Kolodiazhnyi |
Autore | Kolodiazhnyi Oleg I. |
Pubbl/distr/stampa | Weinheim, [Germany] : , : Wiley-VCH, , 1999 |
Descrizione fisica | 1 online resource (569 p.) |
Disciplina |
547.05
547.07 547.070459 |
Soggetto topico |
Ylides
Organophosphorus compounds Organophosphorus compounds - Synthesis |
ISBN |
1-281-84249-4
9786611842499 3-527-61390-0 3-527-61391-9 |
Formato | Materiale a stampa ![]() |
Livello bibliografico | Monografia |
Lingua di pubblicazione | eng |
Nota di contenuto |
Phosphorus Ylides; Contents; 1 Introduction; 1.1 Historiography; 1.2 Types of Phosphorus Ylides and Structure of Book; 1.3 Nornenclature; References; 2 C,P-Carbo-Substituted Phosphorus Ylides; 2.1 Introduction; 2.1.1 Types of C,P-Carbo-Substituted Posphorus Ylides; 2.2 Preparation; 2.2.1 Synthesis from Phosphonium Salts; 2.2.1.1 Dehydrohalogenation of Phosphonium Salts; 2.2.1.2 Synthesis from a-Silyl and a-Stannyl-Substituted Phosphonium Salts; 2.2.1.3 Preparation in Heterogeneous Media; 2.2.1.4 Electrochemical Method; 2.2.1.5 Ultrasound; 2.2.2 Modification of Simple Phosphorus Ylides
2.2.2.1 Acylation2.2.2.2 Alkylation; 2.2.2.3 Arylation; 2.2.3 Addition of Tertiary Phosphines to Compounds Containing Multiple Bonds; 2.2.3.1 Alkenes; 2.2.3.2 Alkynes; 2.2.4 Reaction of Tetracoordinatc Phosphorus Compounds with Multiple-Bonded Compounds; 2.2.5 Modification of the Side-Chain; 2.2.6 Miscellaneous Methods; 2.2.6.1 Formation from Carbenes; 2.2.6.2 Phosphorylation of Cornpounds with an Active Methylene Group; 2.3 Chemical Properties; 2.3.1 Stability; 2.3.2 Transformations Accompanied by Cleavage of the P=C Bond; 2.3.2.1 Thermolysis; 2.3.2.2 Photolysis 2.3.2.3 Oxidation-Industrial Synthesis of B-Carotene2.3.2.4 Reactions with Elemental Sulfur and Selenium; 2.3.2.5 Reduction; 2.3.3.6 Hydrolysis of Ylides; 2.3.2.7 Applications in Organic Synthesis; 2.3.3 Substitution at the Ylidic Carbon Atom; 2.3.3.1 Reactions with Alkylation Reagents; 2.3.3.2 Reactions with Acylation Reagents; 2.3.3.3 Examples in Natural Compound Synthesis; 2.3.4 Reactions with Compounds Containing Multiple Bonds; 2.3.4.1 Compounds Containing Carbon-Carbon Multiple Bonds; 2.3.4.2 Reactions with Compounds Containing Carbon-Heteroatom or Heteroatom-Heteroatom Multiple Bonds 2.3.5 Reactions with 1,3-Dipolar Compounds. Synthesis of Heterocyclic Systems2.3.5.1 Reaction with Aziridines and Azomethine Ylides-Synthesis of Pyrrolines; 2.3.5.2 Oxides of Azomethines; 2.3.5.3 Azides-Synthesis of 1,2, 3-Triazoles; 2.3.5.4 Reaction with Nitrile Oxides. Nitrilimines and Nitrilylides - Synthesis of Pyrazoles and Isoxazoles; References; 3 Cumulene Ylides; 3.1 Introduction; 3.1.1 The Structure of Phosphacumulene Ylides; 3.2 Phosphaketene Ylides; 3.2.1 Chemical Properties; 3.2.2 Dimerization; 3.2.3 Addition of Compounds Bearing a Mobile Hydrogen Atom 3.2.4 [2+2] Cycloaddition Reactions3.2.5 1,3-Dipolar Addition Reactions; 3.2.6 [4+2]-Cycloaddition Reactions; 3.2.7 Miscellaneous Reactions; 3.3 Phosphaketeneacetal Ylides; 3.4 Phosphaallene Ylides and Phosphacumulene Ylides; 3.5 Application in Natural Product Synthesis; 3.6 Carbodiphophoranes; 3.6.1 Structural Studies of Carbodiphosphoranes; References; 4 C-Heterosubstituted Phosphorus Ylides; 4.1 Introduction; 4.2 Phosphorus Ylides Substituted on the a-Carbon by Atoms of Element Groups I-IV; 4.2.1 Ylides Containing Group 1A and IIA Elements; 4.2.2 Ylides Containing Group IIIA Elements 4.2.3 Ylides Containing Group IVA Elements |
Record Nr. | UNISA-996201943103316 |
Kolodiazhnyi Oleg I.
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Weinheim, [Germany] : , : Wiley-VCH, , 1999 | ||
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Lo trovi qui: Univ. di Salerno | ||
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Phosphorus ylides : chemistry and application in organic synthesis / / Oleg I. Kolodiazhnyi |
Autore | Kolodiazhnyi Oleg I. |
Pubbl/distr/stampa | Weinheim, [Germany] : , : Wiley-VCH, , 1999 |
Descrizione fisica | 1 online resource (569 p.) |
Disciplina |
547.05
547.07 547.070459 |
Soggetto topico |
Ylides
Organophosphorus compounds Organophosphorus compounds - Synthesis |
ISBN |
1-281-84249-4
9786611842499 3-527-61390-0 3-527-61391-9 |
Formato | Materiale a stampa ![]() |
Livello bibliografico | Monografia |
Lingua di pubblicazione | eng |
Nota di contenuto |
Phosphorus Ylides; Contents; 1 Introduction; 1.1 Historiography; 1.2 Types of Phosphorus Ylides and Structure of Book; 1.3 Nornenclature; References; 2 C,P-Carbo-Substituted Phosphorus Ylides; 2.1 Introduction; 2.1.1 Types of C,P-Carbo-Substituted Posphorus Ylides; 2.2 Preparation; 2.2.1 Synthesis from Phosphonium Salts; 2.2.1.1 Dehydrohalogenation of Phosphonium Salts; 2.2.1.2 Synthesis from a-Silyl and a-Stannyl-Substituted Phosphonium Salts; 2.2.1.3 Preparation in Heterogeneous Media; 2.2.1.4 Electrochemical Method; 2.2.1.5 Ultrasound; 2.2.2 Modification of Simple Phosphorus Ylides
2.2.2.1 Acylation2.2.2.2 Alkylation; 2.2.2.3 Arylation; 2.2.3 Addition of Tertiary Phosphines to Compounds Containing Multiple Bonds; 2.2.3.1 Alkenes; 2.2.3.2 Alkynes; 2.2.4 Reaction of Tetracoordinatc Phosphorus Compounds with Multiple-Bonded Compounds; 2.2.5 Modification of the Side-Chain; 2.2.6 Miscellaneous Methods; 2.2.6.1 Formation from Carbenes; 2.2.6.2 Phosphorylation of Cornpounds with an Active Methylene Group; 2.3 Chemical Properties; 2.3.1 Stability; 2.3.2 Transformations Accompanied by Cleavage of the P=C Bond; 2.3.2.1 Thermolysis; 2.3.2.2 Photolysis 2.3.2.3 Oxidation-Industrial Synthesis of B-Carotene2.3.2.4 Reactions with Elemental Sulfur and Selenium; 2.3.2.5 Reduction; 2.3.3.6 Hydrolysis of Ylides; 2.3.2.7 Applications in Organic Synthesis; 2.3.3 Substitution at the Ylidic Carbon Atom; 2.3.3.1 Reactions with Alkylation Reagents; 2.3.3.2 Reactions with Acylation Reagents; 2.3.3.3 Examples in Natural Compound Synthesis; 2.3.4 Reactions with Compounds Containing Multiple Bonds; 2.3.4.1 Compounds Containing Carbon-Carbon Multiple Bonds; 2.3.4.2 Reactions with Compounds Containing Carbon-Heteroatom or Heteroatom-Heteroatom Multiple Bonds 2.3.5 Reactions with 1,3-Dipolar Compounds. Synthesis of Heterocyclic Systems2.3.5.1 Reaction with Aziridines and Azomethine Ylides-Synthesis of Pyrrolines; 2.3.5.2 Oxides of Azomethines; 2.3.5.3 Azides-Synthesis of 1,2, 3-Triazoles; 2.3.5.4 Reaction with Nitrile Oxides. Nitrilimines and Nitrilylides - Synthesis of Pyrazoles and Isoxazoles; References; 3 Cumulene Ylides; 3.1 Introduction; 3.1.1 The Structure of Phosphacumulene Ylides; 3.2 Phosphaketene Ylides; 3.2.1 Chemical Properties; 3.2.2 Dimerization; 3.2.3 Addition of Compounds Bearing a Mobile Hydrogen Atom 3.2.4 [2+2] Cycloaddition Reactions3.2.5 1,3-Dipolar Addition Reactions; 3.2.6 [4+2]-Cycloaddition Reactions; 3.2.7 Miscellaneous Reactions; 3.3 Phosphaketeneacetal Ylides; 3.4 Phosphaallene Ylides and Phosphacumulene Ylides; 3.5 Application in Natural Product Synthesis; 3.6 Carbodiphophoranes; 3.6.1 Structural Studies of Carbodiphosphoranes; References; 4 C-Heterosubstituted Phosphorus Ylides; 4.1 Introduction; 4.2 Phosphorus Ylides Substituted on the a-Carbon by Atoms of Element Groups I-IV; 4.2.1 Ylides Containing Group 1A and IIA Elements; 4.2.2 Ylides Containing Group IIIA Elements 4.2.3 Ylides Containing Group IVA Elements |
Record Nr. | UNINA-9910830570903321 |
Kolodiazhnyi Oleg I.
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Weinheim, [Germany] : , : Wiley-VCH, , 1999 | ||
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Lo trovi qui: Univ. Federico II | ||
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