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Advances in multi-photon processes and spectroscopy . Volume 21 / / edited by S.H. Lin, National Chiao-Tung University, Taiwan, Institute of Atomic and Molecular Sciences, Taiwan and Arizona State University, USA, A.A. Villaeys, Institute de Physique et Chimie des Materiaux de Strasbourg, France, Y. Fujimura, Tohoku University, Japan
Advances in multi-photon processes and spectroscopy . Volume 21 / / edited by S.H. Lin, National Chiao-Tung University, Taiwan, Institute of Atomic and Molecular Sciences, Taiwan and Arizona State University, USA, A.A. Villaeys, Institute de Physique et Chimie des Materiaux de Strasbourg, France, Y. Fujimura, Tohoku University, Japan
Pubbl/distr/stampa New Jersey : , : World Scientific, , [2014]
Descrizione fisica 1 online resource (xii, 244 pages) : illustrations (some color)
Disciplina 257
Collana Advances in Multi-Photon Processes and Spectroscopy
Soggetto topico Multiphoton processes
Molecular spectroscopy
ISBN 981-4518-34-4
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto Preface; CONTENTS; 1. Vibrational and Electronic Wavepackets Driven by Strong Field Multiphoton Ionization; 1.1 Introduction; 1.2 Theoretical Concepts; 1.2.1 The time-independent Schrödinger equation and its implications on dynamics; 1.2.2 Spin-orbit coupling and diabatic vs. adiabatic states; 1.2.3 Nuclear time-dependent Schrödinger equation; 1.2.3.1 Second-order differentiator; 1.2.3.2 Split-operator method; 1.2.4 Stark shifts; 1.2.5 Multi- vs. single-photon transitions; 1.2.6 Laser-dressed states; 1.2.7 Photon locking; 1.2.8 Hole burning; 1.2.9 Strong-field ionization
1.3 Computational and experimental details 1.4 Vibrational Wavepackets Created by Multiphoton Ionization; 1.4.1 Phase-dependent dissociation; 1.4.1.1 Photon locking; 1.4.1.2 Hole burning; 1.4.2 Ionization to different ionic states; 1.4.2.1 Preparing electronic wavepackets via SFI; 1.4.2.2 VMI measurements to identify dissociation pathways following SFI; 1.5 Conclusion and Outlook; References; 2. Orientation-Selective Molecular Tunneling Ionization by Phase-Controlled Laser Fields; 1 Introduction; 2 Photoionization Induced by Intense Laser Fields; 2.1 MPI in standard perturbation theory
2.2 Keldysh theory: From MPI to TI2.3 Characteristics of TI; 2.4 Molecular TI; 3 Directionally Asymmetric TI Induced by Phase-controlled Laser Fields; 3.1 Phase-controlled laser fields; 3.2 Directionally asymmetric TI (atoms); 3.3 Directionally asymmetric TI (molecules); 4 Experimental; 5 Results and Discussion; 5.1 Diatomic molecule: CO; 5.1.1 Photo fragment detection; 5.1.2 Photoelectron detection; 5.2 Other molecules; 5.2.1 Nonpolar molecule with asymmetric structure: Br(CH2)2 Cl; 5.2.2 Large molecule: C6H13I; 5.2.3 Systematically changing molecular system: CH3X(X=F,Cl,Br, I)
5.2.4 OCS molecule investigated by nanosecond ω + 2ω laser fields 6 Summary; Acknowledgments; References; 3. Reaction and Ionization of Polyatomic Molecules Induced by Intense Laser Pulses; 1.1 Introduction; 1.2 Ionization Rate of Molecules in Intense Laser Fields; 1.2.1 Theoretical approaches for ionization rates of molecules in intense laser fields; 1.2.2 Experimental measurements of ionization rates of molecules and comparations with theory; 1.3 Fragmentation of Molecules in Intense Laser Fields
1.3.1 Ionization-dissociation of molecules in intense laser fields and statistical theoretical description 1.3.2 Effects of cation absorption on molecular dissociation; 1.4 Dissociative Ionization and Coulombic Explosion of Molecules in Intense Laser Fields; 1.4.1 Dissociative ionization of formic acid molecules; 1.4.2 Coulombic explosion of CH3I; 1.5 Summary and Perspectives; Acknowledgments; References; 4. Ultrafast Internal Conversion of Pyrazine Via Conical Intersection; 1.1 Introduction; 1.2 Pyrazine: Ultrafast S2(1B2u, ππ*) - S1(1B3u, nπ*) Internal Conversion Via Conical Intersection
1.3 Sub-20 fs Deep UV Laser for TRPEI of Pyrazine
Record Nr. UNINA-9910790972903321
New Jersey : , : World Scientific, , [2014]
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui
Advances in multi-photon processes and spectroscopy . Volume 21 / / edited by S.H. Lin, National Chiao-Tung University, Taiwan, Institute of Atomic and Molecular Sciences, Taiwan and Arizona State University, USA, A.A. Villaeys, Institute de Physique et Chimie des Materiaux de Strasbourg, France, Y. Fujimura, Tohoku University, Japan
Advances in multi-photon processes and spectroscopy . Volume 21 / / edited by S.H. Lin, National Chiao-Tung University, Taiwan, Institute of Atomic and Molecular Sciences, Taiwan and Arizona State University, USA, A.A. Villaeys, Institute de Physique et Chimie des Materiaux de Strasbourg, France, Y. Fujimura, Tohoku University, Japan
Pubbl/distr/stampa New Jersey : , : World Scientific, , [2014]
Descrizione fisica 1 online resource (xii, 244 pages) : illustrations (some color)
Disciplina 257
Collana Advances in Multi-Photon Processes and Spectroscopy
Soggetto topico Multiphoton processes
Molecular spectroscopy
ISBN 981-4518-34-4
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto Preface; CONTENTS; 1. Vibrational and Electronic Wavepackets Driven by Strong Field Multiphoton Ionization; 1.1 Introduction; 1.2 Theoretical Concepts; 1.2.1 The time-independent Schrödinger equation and its implications on dynamics; 1.2.2 Spin-orbit coupling and diabatic vs. adiabatic states; 1.2.3 Nuclear time-dependent Schrödinger equation; 1.2.3.1 Second-order differentiator; 1.2.3.2 Split-operator method; 1.2.4 Stark shifts; 1.2.5 Multi- vs. single-photon transitions; 1.2.6 Laser-dressed states; 1.2.7 Photon locking; 1.2.8 Hole burning; 1.2.9 Strong-field ionization
1.3 Computational and experimental details 1.4 Vibrational Wavepackets Created by Multiphoton Ionization; 1.4.1 Phase-dependent dissociation; 1.4.1.1 Photon locking; 1.4.1.2 Hole burning; 1.4.2 Ionization to different ionic states; 1.4.2.1 Preparing electronic wavepackets via SFI; 1.4.2.2 VMI measurements to identify dissociation pathways following SFI; 1.5 Conclusion and Outlook; References; 2. Orientation-Selective Molecular Tunneling Ionization by Phase-Controlled Laser Fields; 1 Introduction; 2 Photoionization Induced by Intense Laser Fields; 2.1 MPI in standard perturbation theory
2.2 Keldysh theory: From MPI to TI2.3 Characteristics of TI; 2.4 Molecular TI; 3 Directionally Asymmetric TI Induced by Phase-controlled Laser Fields; 3.1 Phase-controlled laser fields; 3.2 Directionally asymmetric TI (atoms); 3.3 Directionally asymmetric TI (molecules); 4 Experimental; 5 Results and Discussion; 5.1 Diatomic molecule: CO; 5.1.1 Photo fragment detection; 5.1.2 Photoelectron detection; 5.2 Other molecules; 5.2.1 Nonpolar molecule with asymmetric structure: Br(CH2)2 Cl; 5.2.2 Large molecule: C6H13I; 5.2.3 Systematically changing molecular system: CH3X(X=F,Cl,Br, I)
5.2.4 OCS molecule investigated by nanosecond ω + 2ω laser fields 6 Summary; Acknowledgments; References; 3. Reaction and Ionization of Polyatomic Molecules Induced by Intense Laser Pulses; 1.1 Introduction; 1.2 Ionization Rate of Molecules in Intense Laser Fields; 1.2.1 Theoretical approaches for ionization rates of molecules in intense laser fields; 1.2.2 Experimental measurements of ionization rates of molecules and comparations with theory; 1.3 Fragmentation of Molecules in Intense Laser Fields
1.3.1 Ionization-dissociation of molecules in intense laser fields and statistical theoretical description 1.3.2 Effects of cation absorption on molecular dissociation; 1.4 Dissociative Ionization and Coulombic Explosion of Molecules in Intense Laser Fields; 1.4.1 Dissociative ionization of formic acid molecules; 1.4.2 Coulombic explosion of CH3I; 1.5 Summary and Perspectives; Acknowledgments; References; 4. Ultrafast Internal Conversion of Pyrazine Via Conical Intersection; 1.1 Introduction; 1.2 Pyrazine: Ultrafast S2(1B2u, ππ*) - S1(1B3u, nπ*) Internal Conversion Via Conical Intersection
1.3 Sub-20 fs Deep UV Laser for TRPEI of Pyrazine
Record Nr. UNINA-9910808017203321
New Jersey : , : World Scientific, , [2014]
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui
Advances in multi-photon processes and spectroscopy [[electronic resource] /] / edited by S.H. Lin, A.A. Villaeys, Y. Fujimura
Advances in multi-photon processes and spectroscopy [[electronic resource] /] / edited by S.H. Lin, A.A. Villaeys, Y. Fujimura
Pubbl/distr/stampa Singapore, : World Scientific, 2011
Descrizione fisica 1 online resource (259 p.)
Disciplina 543.0858
543.5
543/.0858
Altri autori (Persone) LinS. H <1937-> (Sheng Hsien)
VillaeysA. A
FujimuraY (Yuichi)
Collana Advances in multi-photon processes and spectroscopy
Soggetto topico Multiphoton processes
Spectrum analysis
Laser spectroscopy
Molecular spectra
Soggetto genere / forma Electronic books.
ISBN 1-283-43377-X
9786613433770
981-4343-99-4
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto CONTENTS; 1. Wave Packet Analysis of Femtosecond Stimulated Raman Spectroscopy K. Niu, B. Zhao, Z. Sun and Soo-Y. Lee; 1. Introduction; 2. Theory; 2.1 Coupled wave theory of FSRS and its limitations; 2.2 Quantum theory of FSRS; 3. Applications, Results and Discussion; 3.1 Analytic results for FSRS from a stationary state with polyatomic harmonic potentials; 3.2 Application to FSRS of Rhodamine 6G; 3.3 Application to the FSRS from a coherent vibrational state of CDCl 3; 3.3.1 Direct fifth-order process; 3.3.2 Cascade processes; 3.3.3 Direct fifth-order and cascade results of CDCl 3
4. Conclusion and outlookAcknowledgements; References; 2. Field-Free Molecular Alignment by Two Femosecond Laser Pulses Chengyin Wu, Hongbing Jiang and Qihuang Gong; 1. Introduction; 2. Theory; 2.1 Creation of rotational wavepacket; 2.2 Characterization of rotational wavepacket; 2.3 Control of rotational wavepacket; 3. Experimental Method; 4. Results and Discussion; 4.1 Manipulation of alignment structures; 4.2 Enhancement of molecular alignment; 4.3 Control of molecular population; 5. Applications of Field-Free Aligned Molecules - Frequency Tuning of Few Cycle Femtosecond Laser Pulses
5.1 Parameters5.2 Simulation; 6. Conclusions; Acknowledgements; References; 3. High-Order Harmonic Generation from C60 Fullerene Plasma T. Ozaki; 1. Introduction; 2. Experimental Set-up; 3. Results and Discussion; 3.1 Observation of high-order harmonics from C fullerenes; 3.2 Influence of various experimental parameters on the HHG efficiency in fullerene plasma; 3.3 Simulations of harmonic spectra from C fullerenes; 3.4 Discussions; 4. Conclusions; References
4. Attosecond Pulse Generation, Characterization and Application Shouyuan Chen, Steve Gilbertson, He Wang, Michael Chini, Kun Zhao, Sabih Khan, Yi Wu, and Zenghu Chang1. Introduction; 2. Ultrafast Laser Development and CE Phase Stabilization for Attosecond Pulse Generation; 2.1 CE phase drift caused by the grating drift in stretcher and compressor; 2.2 CE phase stabilization of multi-pass and regenerative amplifiers; 3. Attosecond Gating Technology; 3.1 Two-color gating; 3.2 Polarization gating; 3.3 Double optical gating; 3.4 Generalized double optical gating; 3.5 DOG and GDOG optics
4. Attosecond Pulse Measurement and Characterization4.1 Attosecond streak camera; 4.2 Frequency-resolved optical gating for complete reconstruction of attosecond bursts; 4.3 Phase retrieval by omega oscillation filtering; 5. Application of Attosecond Pulse; 5.1 Study of Helium autoionization by attosecond streaking; 5.2 Time resolved spectroscopy study of Argon; 6. Summary and Outlook; References; 5. Near-Field Imaging of Optical-Field Structures and Plasmon Wave Functions in Metal Nanostructures Hiromi Okamoto and Kohei Imura; 1. Introduction
2. What can be Observed by Near-Field Optical Imaging?
Record Nr. UNINA-9910464497303321
Singapore, : World Scientific, 2011
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui
Advances in multi-photon processes and spectroscopy [[electronic resource] /] / edited by S.H. Lin, A.A. Villaeys, Y. Fujimura
Advances in multi-photon processes and spectroscopy [[electronic resource] /] / edited by S.H. Lin, A.A. Villaeys, Y. Fujimura
Pubbl/distr/stampa Singapore, : World Scientific, 2011
Descrizione fisica 1 online resource (259 p.)
Disciplina 543.0858
543.5
543/.0858
Altri autori (Persone) LinS. H <1937-> (Sheng Hsien)
VillaeysA. A
FujimuraY (Yuichi)
Collana Advances in multi-photon processes and spectroscopy
Soggetto topico Multiphoton processes
Spectrum analysis
Laser spectroscopy
Molecular spectra
ISBN 1-283-43377-X
9786613433770
981-4343-99-4
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto CONTENTS; 1. Wave Packet Analysis of Femtosecond Stimulated Raman Spectroscopy K. Niu, B. Zhao, Z. Sun and Soo-Y. Lee; 1. Introduction; 2. Theory; 2.1 Coupled wave theory of FSRS and its limitations; 2.2 Quantum theory of FSRS; 3. Applications, Results and Discussion; 3.1 Analytic results for FSRS from a stationary state with polyatomic harmonic potentials; 3.2 Application to FSRS of Rhodamine 6G; 3.3 Application to the FSRS from a coherent vibrational state of CDCl 3; 3.3.1 Direct fifth-order process; 3.3.2 Cascade processes; 3.3.3 Direct fifth-order and cascade results of CDCl 3
4. Conclusion and outlookAcknowledgements; References; 2. Field-Free Molecular Alignment by Two Femosecond Laser Pulses Chengyin Wu, Hongbing Jiang and Qihuang Gong; 1. Introduction; 2. Theory; 2.1 Creation of rotational wavepacket; 2.2 Characterization of rotational wavepacket; 2.3 Control of rotational wavepacket; 3. Experimental Method; 4. Results and Discussion; 4.1 Manipulation of alignment structures; 4.2 Enhancement of molecular alignment; 4.3 Control of molecular population; 5. Applications of Field-Free Aligned Molecules - Frequency Tuning of Few Cycle Femtosecond Laser Pulses
5.1 Parameters5.2 Simulation; 6. Conclusions; Acknowledgements; References; 3. High-Order Harmonic Generation from C60 Fullerene Plasma T. Ozaki; 1. Introduction; 2. Experimental Set-up; 3. Results and Discussion; 3.1 Observation of high-order harmonics from C fullerenes; 3.2 Influence of various experimental parameters on the HHG efficiency in fullerene plasma; 3.3 Simulations of harmonic spectra from C fullerenes; 3.4 Discussions; 4. Conclusions; References
4. Attosecond Pulse Generation, Characterization and Application Shouyuan Chen, Steve Gilbertson, He Wang, Michael Chini, Kun Zhao, Sabih Khan, Yi Wu, and Zenghu Chang1. Introduction; 2. Ultrafast Laser Development and CE Phase Stabilization for Attosecond Pulse Generation; 2.1 CE phase drift caused by the grating drift in stretcher and compressor; 2.2 CE phase stabilization of multi-pass and regenerative amplifiers; 3. Attosecond Gating Technology; 3.1 Two-color gating; 3.2 Polarization gating; 3.3 Double optical gating; 3.4 Generalized double optical gating; 3.5 DOG and GDOG optics
4. Attosecond Pulse Measurement and Characterization4.1 Attosecond streak camera; 4.2 Frequency-resolved optical gating for complete reconstruction of attosecond bursts; 4.3 Phase retrieval by omega oscillation filtering; 5. Application of Attosecond Pulse; 5.1 Study of Helium autoionization by attosecond streaking; 5.2 Time resolved spectroscopy study of Argon; 6. Summary and Outlook; References; 5. Near-Field Imaging of Optical-Field Structures and Plasmon Wave Functions in Metal Nanostructures Hiromi Okamoto and Kohei Imura; 1. Introduction
2. What can be Observed by Near-Field Optical Imaging?
Record Nr. UNINA-9910788957603321
Singapore, : World Scientific, 2011
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui
Advances in multi-photon processes and spectroscopy [[electronic resource] ] . Volume 18 / / edited by S.H. Lin, A.A. Villaeys, Y. Fujimura
Advances in multi-photon processes and spectroscopy [[electronic resource] ] . Volume 18 / / edited by S.H. Lin, A.A. Villaeys, Y. Fujimura
Pubbl/distr/stampa Hackensack, NJ, : World Scientific, c2008
Descrizione fisica 1 online resource (304 p.)
Disciplina 543.085
543.0858
543/.0858
Altri autori (Persone) FujimuraY (Yuichi)
LinS. H <1937-> (Sheng Hsien)
VillaeysA. A
Collana Advances in Multi-Photon Processes and Spectroscopy
Soggetto topico Molecular spectra
Multiphoton processes
Spectrum analysis
Soggetto genere / forma Electronic books.
ISBN 1-281-93399-6
9786611933999
981-279-174-4
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto Contents; Preface; 1. Nonlinear Optics for Characterizing XUV/Soft X-ray High-order Harmonic Fields in Attosecond Regime Yasuo Nabekawa and Katsumi Midorikawa; 1. Introduction; 1.1. Nonlinear phenomena in XUV/soft X-ray region for ultrafast optics; 1.2. Autocorrelation measurement; 2. Generation of Intense Harmonic Fields; 2.1. Single atom response; 2.2. Propagation of the harmonic fields with pumping laser field: Phase matching; 2.3. Development of intense high-order harmonic generator; 3. Two-Photon Double Ionization; 4. Measurement of Attosecond Pulse Train with Two-Photon ATI
5. Interferometric Autocorrelation of APT with Two-Photon Coulomb Explosion 5.1. Similarity of APT with mode-locked laser pulses; 5.2. Why do we need interferometric autocorrelation?; 5.3. Two-photon Coulomb explosion; 5.4. Interferometric autocorrelation; 6. Summary and Prospects; Acknowledgements; References; 2. Signatures of Molecular Structure and Dynamics in High-Order Harmonic Generation Manfred Lein and Ciprian C. Chiril ̆a; 1. Introduction; 2. Theory of High-Order Harmonic Generation; 2.1. Basic theory; 2.2. Three-step model; 2.3. The strong-field approximation
2.4. Odd and even harmonics3. Influence of Molecular Structure on HHG; 3.1. Ionization step; 3.2. Recombination step; 4. Dynamical Effects; 5. Conclusions; Acknowledgments; References; 3. Molecular Manipulation Techniques and Their Applications Hirofumi Sakai; 1. Introduction; 2. Theoretical Background; 3. Molecular Orientation with Combined Electrostatic and Intense, Nonresonant Laser Fields; 3.1. One-dimensional molecular orientation; 3.2. Three-dimensional molecular orientation; 4. Applications with a Sample of Aligned Molecules
4.1. Optimal control of multiphoton ionization processes in aligned I2 molecules with time-dependent polarization pulses 4.2. High-order harmonic generation from aligned molecules; 5. Summary and Outlook; Acknowledgments; References; 4. Sum Frequency Generation: An Introduction with Recent Developments and Current Issues Mary Jane Shultz; 1. Introduction; 2. Electric Fields and Orientation Factors; 2.1. Fresnel factors and propagation direction; 2.2. Orientation factors; 2.2.1. Simplification of the orientation tensor; 2.3. Observed intensity; 2.3.1. Molecular examples; 3. Recent Developments
3.1. Absolute orientation determination with a reference 3.2. Orthogonal resonances; 3.3. Null angle; 3.3.1. Visible angle null, VAN; 3.3.2. Polarization angle null, PAN; 3.3.3. Connection with previous work; 3.3.4. Example; 4. Current Issues in Sum Frequency Generation; 4.1. Interfacial optical constants and bulk contributions; 4.2. Collective modes - a theoretical challenge; 4.3. Probe depth; 4.4. Nanoparticle SFG; 4.5. Time resolution; 4.6. Surface 2D imaging; 5. Selected Results; 5.1. Ions at aqueous surfaces: The case for surface H3O+; 5.2. Interactions at nanostructured interfaces
6. Summary
Record Nr. UNINA-9910453555003321
Hackensack, NJ, : World Scientific, c2008
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui
Advances in multi-photon processes and spectroscopy [[electronic resource] ] . Volume 18 / / edited by S.H. Lin, A.A. Villaeys, Y. Fujimura
Advances in multi-photon processes and spectroscopy [[electronic resource] ] . Volume 18 / / edited by S.H. Lin, A.A. Villaeys, Y. Fujimura
Pubbl/distr/stampa Hackensack, NJ, : World Scientific, c2008
Descrizione fisica 1 online resource (304 p.)
Disciplina 543.085
543.0858
543/.0858
Altri autori (Persone) FujimuraY (Yuichi)
LinS. H <1937-> (Sheng Hsien)
VillaeysA. A
Collana Advances in Multi-Photon Processes and Spectroscopy
Soggetto topico Molecular spectra
Multiphoton processes
Spectrum analysis
ISBN 1-281-93399-6
9786611933999
981-279-174-4
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto Contents; Preface; 1. Nonlinear Optics for Characterizing XUV/Soft X-ray High-order Harmonic Fields in Attosecond Regime Yasuo Nabekawa and Katsumi Midorikawa; 1. Introduction; 1.1. Nonlinear phenomena in XUV/soft X-ray region for ultrafast optics; 1.2. Autocorrelation measurement; 2. Generation of Intense Harmonic Fields; 2.1. Single atom response; 2.2. Propagation of the harmonic fields with pumping laser field: Phase matching; 2.3. Development of intense high-order harmonic generator; 3. Two-Photon Double Ionization; 4. Measurement of Attosecond Pulse Train with Two-Photon ATI
5. Interferometric Autocorrelation of APT with Two-Photon Coulomb Explosion 5.1. Similarity of APT with mode-locked laser pulses; 5.2. Why do we need interferometric autocorrelation?; 5.3. Two-photon Coulomb explosion; 5.4. Interferometric autocorrelation; 6. Summary and Prospects; Acknowledgements; References; 2. Signatures of Molecular Structure and Dynamics in High-Order Harmonic Generation Manfred Lein and Ciprian C. Chiril ̆a; 1. Introduction; 2. Theory of High-Order Harmonic Generation; 2.1. Basic theory; 2.2. Three-step model; 2.3. The strong-field approximation
2.4. Odd and even harmonics3. Influence of Molecular Structure on HHG; 3.1. Ionization step; 3.2. Recombination step; 4. Dynamical Effects; 5. Conclusions; Acknowledgments; References; 3. Molecular Manipulation Techniques and Their Applications Hirofumi Sakai; 1. Introduction; 2. Theoretical Background; 3. Molecular Orientation with Combined Electrostatic and Intense, Nonresonant Laser Fields; 3.1. One-dimensional molecular orientation; 3.2. Three-dimensional molecular orientation; 4. Applications with a Sample of Aligned Molecules
4.1. Optimal control of multiphoton ionization processes in aligned I2 molecules with time-dependent polarization pulses 4.2. High-order harmonic generation from aligned molecules; 5. Summary and Outlook; Acknowledgments; References; 4. Sum Frequency Generation: An Introduction with Recent Developments and Current Issues Mary Jane Shultz; 1. Introduction; 2. Electric Fields and Orientation Factors; 2.1. Fresnel factors and propagation direction; 2.2. Orientation factors; 2.2.1. Simplification of the orientation tensor; 2.3. Observed intensity; 2.3.1. Molecular examples; 3. Recent Developments
3.1. Absolute orientation determination with a reference 3.2. Orthogonal resonances; 3.3. Null angle; 3.3.1. Visible angle null, VAN; 3.3.2. Polarization angle null, PAN; 3.3.3. Connection with previous work; 3.3.4. Example; 4. Current Issues in Sum Frequency Generation; 4.1. Interfacial optical constants and bulk contributions; 4.2. Collective modes - a theoretical challenge; 4.3. Probe depth; 4.4. Nanoparticle SFG; 4.5. Time resolution; 4.6. Surface 2D imaging; 5. Selected Results; 5.1. Ions at aqueous surfaces: The case for surface H3O+; 5.2. Interactions at nanostructured interfaces
6. Summary
Record Nr. UNINA-9910782342703321
Hackensack, NJ, : World Scientific, c2008
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui
Advances in multi-photon processes and spectroscopy [[electronic resource] ] . Volume 17 / / edited by S.H. Lin, A.A. Vilaeys, Y. Fujimura
Advances in multi-photon processes and spectroscopy [[electronic resource] ] . Volume 17 / / edited by S.H. Lin, A.A. Vilaeys, Y. Fujimura
Pubbl/distr/stampa Hackensack, NJ, : World Scientific, c2006
Descrizione fisica 1 online resource (228 p.)
Disciplina 543.8
Altri autori (Persone) FujimuraY (Yuichi)
LinS. H <1937-> (Sheng Hsien)
VillaeysA. A
Collana Advances in Multi-Photon Processes and Spectroscopy
Soggetto topico Molecular spectra
Multiphoton processes
Spectrum analysis
Soggetto genere / forma Electronic books.
ISBN 1-281-90898-3
9786611908980
981-270-715-8
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto CONTENTS; Preface; 1 Probing Orbital Symmetries and Ionization Dynamics of Simple Molecules With Femtosecond Laser Pulses C. D. Lin and X. M. Tong; 1.1. Introduction; 1.2. Probing Molecular Orbital Symmetry with Sub-10 fs Laser Pulses; 1.2.1. Molecular tunneling ionization theory; 1.2.2. Alignment dependence of tunneling ionization rates and the symmetry of molecular orbitals; 1.3. Attosecond Molecular Clocks: Time-Resolved Double Ionization Dynamics of H2 and D2 Molecules; 1.3.1. Dynamics of double ionization of H2 by femtosecond lasers
1.3.2. Theory of double ionization of H2 by femtosecond lasers: rescattering region 1.3.3. Control the time sequence of double ionization by tuning laser parameters; 1.4. Probing Nonclassical Vibrational Wave Packets on Two Potential Surfaces; 1.5. Summary and Discussion; Acknowledgments; References; 2 Generalization and Application to Molecular Systems of Keldysh's Atomic Photoionization Theory K. Mishima, K. Nagaya, M. Hayashi, S. H. Lin and E. W. Schlag; 2.1. General Introduction; 2.2. Original Atomic Keldysh Theory; 2.3. Generalization of the Original Atomic Keldysh Theory
2.3.1. Introduction 2.3.2. Theory-atomic case; 2.3.3. Theory-diatomic molecule case; 2.3.4. Results and discussion; 2.4. Coulomb Correction of the Atomic Keldysh Theory; 2.4.1. Introduction; 2.4.2. Theory; 2.4.3. Results and discussion; 2.5. Application to Large Polyatomic Molecules; 2.5.1. Introduction; 2.5.2. Theory; 2.5.2.1. Molecular Coulomb-corrected Volkov function of electron; 2.5.2.2. Photoionization rate of spatially aligned molecules in the linearly polarized electric field; 2.5.3. Computational method - ab initio calculation; 2.5.4. Numerical results and discussion
2.5.4.1. Ab initio calculation 2.5.4.2. Photoionization rates of all-trans polyacetylene radicals (CnHn+2, n = 3, 5, 7, 9, 13, 27); 2.6. Extension of the Atomic Keldysh Theory to Molecular Photoionization Processes; 2.6.1. Introduction; 2.6.2. Theory; 2.6.3. Computational methods; 2.6.3.1. Ab initio calculation; 2.6.3.2. Calculation of Franck-Condon factors; 2.6.4. Numerical results and discussion; 2.6.5. Introduction; 2.6.6. Theory; 2.6.7. Computational methods; 2.6.7.1. Ab initio calculation; 2.6.7.2. Calculation of potential energy curves and Franck-Condon factors
2.6.8. Numerical results and discussion 2.7. Towards the Realization of the Quantum Chemistry Approach to Tunneling Photoionization Processes in Strong Laser Fields; 2.8. Ab Initio/RRKM Approach to the Elucidation of the Mechanism of Photoionization and Photodissociation of Molecules in Intense Laser Fields; 2.9. Conclusion; Acknowledgments; Appendix; Appendix A. Saddle-Point Method for Integrals with a Singularity; Appendix B. Compact Forms of L(p) Defined by Eq. (64); Appendix C. Definition of N(r, w, I0, I0, B,C) in Eqs. (66) and (79)
Appendix D. Definition of N(r,r,w, I0, A, B) and Integrated Form of Eq. (121)
Record Nr. UNINA-9910453700503321
Hackensack, NJ, : World Scientific, c2006
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui
Advances in multi-photon processes and spectroscopy [[electronic resource] ] . Volume 17 / / edited by S.H. Lin, A.A. Vilaeys, Y. Fujimura
Advances in multi-photon processes and spectroscopy [[electronic resource] ] . Volume 17 / / edited by S.H. Lin, A.A. Vilaeys, Y. Fujimura
Pubbl/distr/stampa Hackensack, NJ, : World Scientific, c2006
Descrizione fisica 1 online resource (228 p.)
Disciplina 543.8
Altri autori (Persone) FujimuraY (Yuichi)
LinS. H <1937-> (Sheng Hsien)
VillaeysA. A
Collana Advances in Multi-Photon Processes and Spectroscopy
Soggetto topico Molecular spectra
Multiphoton processes
Spectrum analysis
ISBN 1-281-90898-3
9786611908980
981-270-715-8
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto CONTENTS; Preface; 1 Probing Orbital Symmetries and Ionization Dynamics of Simple Molecules With Femtosecond Laser Pulses C. D. Lin and X. M. Tong; 1.1. Introduction; 1.2. Probing Molecular Orbital Symmetry with Sub-10 fs Laser Pulses; 1.2.1. Molecular tunneling ionization theory; 1.2.2. Alignment dependence of tunneling ionization rates and the symmetry of molecular orbitals; 1.3. Attosecond Molecular Clocks: Time-Resolved Double Ionization Dynamics of H2 and D2 Molecules; 1.3.1. Dynamics of double ionization of H2 by femtosecond lasers
1.3.2. Theory of double ionization of H2 by femtosecond lasers: rescattering region 1.3.3. Control the time sequence of double ionization by tuning laser parameters; 1.4. Probing Nonclassical Vibrational Wave Packets on Two Potential Surfaces; 1.5. Summary and Discussion; Acknowledgments; References; 2 Generalization and Application to Molecular Systems of Keldysh's Atomic Photoionization Theory K. Mishima, K. Nagaya, M. Hayashi, S. H. Lin and E. W. Schlag; 2.1. General Introduction; 2.2. Original Atomic Keldysh Theory; 2.3. Generalization of the Original Atomic Keldysh Theory
2.3.1. Introduction 2.3.2. Theory-atomic case; 2.3.3. Theory-diatomic molecule case; 2.3.4. Results and discussion; 2.4. Coulomb Correction of the Atomic Keldysh Theory; 2.4.1. Introduction; 2.4.2. Theory; 2.4.3. Results and discussion; 2.5. Application to Large Polyatomic Molecules; 2.5.1. Introduction; 2.5.2. Theory; 2.5.2.1. Molecular Coulomb-corrected Volkov function of electron; 2.5.2.2. Photoionization rate of spatially aligned molecules in the linearly polarized electric field; 2.5.3. Computational method - ab initio calculation; 2.5.4. Numerical results and discussion
2.5.4.1. Ab initio calculation 2.5.4.2. Photoionization rates of all-trans polyacetylene radicals (CnHn+2, n = 3, 5, 7, 9, 13, 27); 2.6. Extension of the Atomic Keldysh Theory to Molecular Photoionization Processes; 2.6.1. Introduction; 2.6.2. Theory; 2.6.3. Computational methods; 2.6.3.1. Ab initio calculation; 2.6.3.2. Calculation of Franck-Condon factors; 2.6.4. Numerical results and discussion; 2.6.5. Introduction; 2.6.6. Theory; 2.6.7. Computational methods; 2.6.7.1. Ab initio calculation; 2.6.7.2. Calculation of potential energy curves and Franck-Condon factors
2.6.8. Numerical results and discussion 2.7. Towards the Realization of the Quantum Chemistry Approach to Tunneling Photoionization Processes in Strong Laser Fields; 2.8. Ab Initio/RRKM Approach to the Elucidation of the Mechanism of Photoionization and Photodissociation of Molecules in Intense Laser Fields; 2.9. Conclusion; Acknowledgments; Appendix; Appendix A. Saddle-Point Method for Integrals with a Singularity; Appendix B. Compact Forms of L(p) Defined by Eq. (64); Appendix C. Definition of N(r, w, I0, I0, B,C) in Eqs. (66) and (79)
Appendix D. Definition of N(r,r,w, I0, A, B) and Integrated Form of Eq. (121)
Record Nr. UNINA-9910782233803321
Hackensack, NJ, : World Scientific, c2006
Materiale a stampa
Lo trovi qui: Univ. Federico II
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Advances in multi-photon processes and spectroscopy . Volume 15 [[electronic resource] /] / edited by S. H. Lin, A. A. Villaeys, Y. Fujimura
Advances in multi-photon processes and spectroscopy . Volume 15 [[electronic resource] /] / edited by S. H. Lin, A. A. Villaeys, Y. Fujimura
Pubbl/distr/stampa Singapore, : World Scientific, c2003
Descrizione fisica 1 online resource (383 p.)
Disciplina 543.0858
Altri autori (Persone) LinS. H <1937-> (Sheng Hsien)
VillaeysA. A
FujimuraY (Yuichi)
Collana Advances in multi-photon processes and spectroscopy
Soggetto topico Laser spectroscopy
Molecular spectra
Multiphoton processes
Spectrum analysis
Soggetto genere / forma Electronic books.
ISBN 1-281-93577-8
9786611935771
981-279-537-5
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto Preface; Contents; Part One: Polarizabilities and Hyperpolarizabilities of Dendritic Systems; Polarizabilities and Hyperpolarizabilities of Dendritic Systems; Abstract; 1. Introduction; 2. Polarizabilities and Hyperpolarizabilities of Dendritic Aggregate Systems; 2.1. Aggregate Models; 2.2. Density Matrix Formalism for Molecular Aggregate under Time-Dependent Electric Field; 2.3. Nonperturbative (Hyper)polarizabilities and Their Partition into the Contribution of Exciton Generation; 2.4. Off-Resonant Polarizabilities of Dendritic Aggregates
2.5. Off-Resonant Second Hyperpolarizabilities of Dendritic Aggregates 2.6. Near-Resonant Second Hyperpolarizabilities of Dendritic Aggregates; 2.7. Summary; 3. Polarizabilities and Hyperpolarizabilities of Dendrimers; 3.1. Cayley-Tree-Type Dendrimers with TT-Conjugation; 3.2. Finite-Field Approach to Static (Hyper)polarizabilities; 3.3. Hyperpolarizability Density Analysis; 3.4. Size Dependencies of a and yof Oligomer Models for Dendron Parts; 3.5. Second Hyperpolarizabilities of Cayley-Tree-Type Phenylacetylene Dendrimers; 3.6. Summary; 4. Extensions of Models and Analysis
4.1. Master Equation Approach Involving Explicit Exciton-Phonon Coupling 4.2. Analytical Expression of Hyperpolarizability Density; 4.3. Summary; 5. Concluding Remarks; Acknowledgments; References; Part Two: Molecules in Intense Laser Fields: Nonlinear Multiphoton Spectroscopy and Near-Femtosecond To Sub-Femtosecond (Attosecond) Dynamics; Molecules In Intense Laser Fields: Nonlinear Multiphoton Spectroscopy And Near-Femtosecond To Sub-Femtosecond (Attosecond) Dynamics; 1 Introduction; 2 Numerical Methods; 3 Charge Resonance Enhanced Ionization and Quasistatic Models: One-Electron Systems
4 Two-Electron Systems 5 Adiabatic State Formalism; 6 Adiabatic State Population Analysis; 7 Transfer Matrix Formalism; 8 High-Frequency Limit; 9 Conclusion; Acknowledgments; References; Part Three: Ultrafast Dynamics and non-Markovian Processes in Four-Photon Spectroscopy; Ultrafast Dynamics and non-Markovian Processes in Four-Photon Spectroscopy; 1 Introduction; 2 Hamiltonian of chromofore molecule in solvent and basic methods of the resonance four-photon spectroscopy; 3 Calculation of nonlinear polarization; 4 Stochastic models in transient RFPS
4.1 Non-Markovian relaxation effects in two-pulse RFPS with Gaussian random modulation of optical transition frequency 4.2 Transient four-photon spectroscopy of near or overlapping resonances in the presence of spectral exchange; 4.3 Non-Markovian relaxation effects in three-pulse RFPS; 5 Non-Markovian theory of steady-state RFPS; 5.1 Introduction and the cubic susceptibility in the case of Gaussian-Markovian random modulation of an electronic transition; 5.2 Model for frequency modulation of electronic transition of complex molecule in solution
5.3 Cubic susceptibility for detunings larger than reciprocal correlation time
Record Nr. UNINA-9910454357803321
Singapore, : World Scientific, c2003
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui
Advances in multi-photon processes and spectroscopy . Volume 15 [[electronic resource] /] / edited by S. H. Lin, A. A. Villaeys, Y. Fujimura
Advances in multi-photon processes and spectroscopy . Volume 15 [[electronic resource] /] / edited by S. H. Lin, A. A. Villaeys, Y. Fujimura
Pubbl/distr/stampa Singapore, : World Scientific, c2003
Descrizione fisica 1 online resource (383 p.)
Disciplina 543.0858
Altri autori (Persone) LinS. H <1937-> (Sheng Hsien)
VillaeysA. A
FujimuraY (Yuichi)
Collana Advances in multi-photon processes and spectroscopy
Soggetto topico Laser spectroscopy
Molecular spectra
Multiphoton processes
Spectrum analysis
ISBN 1-281-93577-8
9786611935771
981-279-537-5
Formato Materiale a stampa
Livello bibliografico Monografia
Lingua di pubblicazione eng
Nota di contenuto Preface; Contents; Part One: Polarizabilities and Hyperpolarizabilities of Dendritic Systems; Polarizabilities and Hyperpolarizabilities of Dendritic Systems; Abstract; 1. Introduction; 2. Polarizabilities and Hyperpolarizabilities of Dendritic Aggregate Systems; 2.1. Aggregate Models; 2.2. Density Matrix Formalism for Molecular Aggregate under Time-Dependent Electric Field; 2.3. Nonperturbative (Hyper)polarizabilities and Their Partition into the Contribution of Exciton Generation; 2.4. Off-Resonant Polarizabilities of Dendritic Aggregates
2.5. Off-Resonant Second Hyperpolarizabilities of Dendritic Aggregates 2.6. Near-Resonant Second Hyperpolarizabilities of Dendritic Aggregates; 2.7. Summary; 3. Polarizabilities and Hyperpolarizabilities of Dendrimers; 3.1. Cayley-Tree-Type Dendrimers with TT-Conjugation; 3.2. Finite-Field Approach to Static (Hyper)polarizabilities; 3.3. Hyperpolarizability Density Analysis; 3.4. Size Dependencies of a and yof Oligomer Models for Dendron Parts; 3.5. Second Hyperpolarizabilities of Cayley-Tree-Type Phenylacetylene Dendrimers; 3.6. Summary; 4. Extensions of Models and Analysis
4.1. Master Equation Approach Involving Explicit Exciton-Phonon Coupling 4.2. Analytical Expression of Hyperpolarizability Density; 4.3. Summary; 5. Concluding Remarks; Acknowledgments; References; Part Two: Molecules in Intense Laser Fields: Nonlinear Multiphoton Spectroscopy and Near-Femtosecond To Sub-Femtosecond (Attosecond) Dynamics; Molecules In Intense Laser Fields: Nonlinear Multiphoton Spectroscopy And Near-Femtosecond To Sub-Femtosecond (Attosecond) Dynamics; 1 Introduction; 2 Numerical Methods; 3 Charge Resonance Enhanced Ionization and Quasistatic Models: One-Electron Systems
4 Two-Electron Systems 5 Adiabatic State Formalism; 6 Adiabatic State Population Analysis; 7 Transfer Matrix Formalism; 8 High-Frequency Limit; 9 Conclusion; Acknowledgments; References; Part Three: Ultrafast Dynamics and non-Markovian Processes in Four-Photon Spectroscopy; Ultrafast Dynamics and non-Markovian Processes in Four-Photon Spectroscopy; 1 Introduction; 2 Hamiltonian of chromofore molecule in solvent and basic methods of the resonance four-photon spectroscopy; 3 Calculation of nonlinear polarization; 4 Stochastic models in transient RFPS
4.1 Non-Markovian relaxation effects in two-pulse RFPS with Gaussian random modulation of optical transition frequency 4.2 Transient four-photon spectroscopy of near or overlapping resonances in the presence of spectral exchange; 4.3 Non-Markovian relaxation effects in three-pulse RFPS; 5 Non-Markovian theory of steady-state RFPS; 5.1 Introduction and the cubic susceptibility in the case of Gaussian-Markovian random modulation of an electronic transition; 5.2 Model for frequency modulation of electronic transition of complex molecule in solution
5.3 Cubic susceptibility for detunings larger than reciprocal correlation time
Record Nr. UNINA-9910782286603321
Singapore, : World Scientific, c2003
Materiale a stampa
Lo trovi qui: Univ. Federico II
Opac: Controlla la disponibilità qui