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Chemical Complexity : Self-Organization Processes in Molecular Systems / / by Alexander S. Mikhailov, Gerhard Ertl
| Chemical Complexity : Self-Organization Processes in Molecular Systems / / by Alexander S. Mikhailov, Gerhard Ertl |
| Autore | Mikhailov Alexander S |
| Edizione | [1st ed. 2017.] |
| Pubbl/distr/stampa | Cham : , : Springer International Publishing : , : Imprint : Springer, , 2017 |
| Descrizione fisica | 1 online resource (209 pages) |
| Disciplina | 547.2 |
| Collana | The Frontiers Collection |
| Soggetto topico |
Chemistry, Physical and theoretical
Statistical physics Computational complexity Systems biology Biological systems Materials—Surfaces Thin films Physical Chemistry Applications of Nonlinear Dynamics and Chaos Theory Complexity Systems Biology Surfaces and Interfaces, Thin Films |
| ISBN | 3-319-57377-2 |
| Formato | Materiale a stampa  |
| Livello bibliografico | Monografia |
| Lingua di pubblicazione | eng |
| Nota di contenuto | Self-organization vs. self-assembly -- Thermodynamics of open systems -- The Turing instability -- Waves in the heart -- The Belousov-Zhabotinsky reaction -- Surface catalysis -- Corrosion of steels -- Nonequilibrium soft matter -- Phase transitions in reactive systems -- Self-organization in biological cells -- Protein machines and molecular motors -- Active propulsion on microscales -- Oscillators and synchronization phenomena -- Chemical chaos -- Network problems -- Design and control of self-organizing systems -- Open problems and application perspectives. |
| Record Nr. | UNINA-9910741200403321 |
Mikhailov Alexander S
|
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| Cham : , : Springer International Publishing : , : Imprint : Springer, , 2017 | ||
| Materiale a stampa | ||
| Lo trovi qui: Univ. Federico II | ||
| ||
Engineering of chemical complexity [[electronic resource] /] / editors, Alexander S. Mikhailov, Gerhard Ertl
| Engineering of chemical complexity [[electronic resource] /] / editors, Alexander S. Mikhailov, Gerhard Ertl |
| Pubbl/distr/stampa | Singapore ; ; Hackensack, NJ, : World Scientific, c2013 |
| Descrizione fisica | 1 online resource (413 p.) |
| Disciplina |
658.00952
660 |
| Altri autori (Persone) |
MikhailovA. S <1950-> (Alexander S.)
ErtlG (Gerhard) |
| Collana | World Scientific lecture notes in complex systems |
| Soggetto topico |
Chemistry - Mathematics
Chaotic behavior in systems |
| Soggetto genere / forma | Electronic books. |
| ISBN |
1-283-97146-1
981-4390-46-1 |
| Formato | Materiale a stampa |
| Livello bibliografico | Monografia |
| Lingua di pubblicazione | eng |
| Nota di contenuto |
CONTENTS; Preface; PART I INTRODUCTION; 1. Analysis, Design and Control of Complex Chemical Systems Alexander S. Mikhailov and Gerhard Ertl; 1. Introduction; 2. A Brief Historical Overview; 3. Recent Developments and Open Perspectives; References; PART II SINGLE MOLECULES, NANOSCALE PHENOMENA AND ACTIVE PARTICLES; 2. Imaging and Manipulation of Single Molecules by Scanning Tunneling Microscopy Leonhard Grill; 1. Introduction; 2. Imaging and Spectroscopy of Single Molecules; 2.1. Imaging single molecules; 2.2. Chemical identification by spectroscopy; 2.3. Imaging of diffusion processes
3. Manipulation of Single Molecules3.1. Manipulation without bias voltage; 3.2. Electron-induced manipulation; 3.3. Electric-field induced manipulation; 3.4. Lateral manipulation: Hopping vs rolling; 3.5. Vertical manipulation: Pulling single molecules from a surface; Acknowledgments; References; 3. Self-Organization at the Nanoscale in Far-From- Equilibrium Surface Reactions and Copolymerizations Pierre Gaspard; 1. Introduction; 2. Fundamental Aspects of Nonequilibrium Nanosystems; 2.1. Structure and function of nanosystems; 2.2. Out-of-equilibrium directionality of fluctuating currents 2.3. Thermodynamic origins of dynamical order3. Heterogeneous Catalytic Reactions in High Electric Fields; 3.1. Surface conditions in FEM and FIM; 3.2. Adsorption-desorption kinetics; 3.3. Surface oxides of rhodium; 3.4. The H2-O2/Rh system; 3.4.1. Kinetic equations; 3.4.2. Bistability; 3.4.3. Oscillations; 3.5. Self-organization at the nanoscale; 4. Copolymerization processes; 4.1. Information processing at the molecular scale; 4.2. Thermodynamics of free copolymerization; 4.3. Thermodynamics of copolymerization with a template; 4.4. The case of DNA replication 5. Conclusions and PerspectivesAcknowledgments; References; 4. Single Molecule and Collective Dynamics of Motor Protein Coupled with Mechano-Sensitive Chemical Reaction Mitsuhiro Iwaki, Lorenzo Marcucci, Yuichi Togashi and Toshio Yanagida; 1. What is a Motor Protein?; 2. Measurement of Myosin at the Single Molecule Level; 3. Mechanosensitivity of ATP Hydrolysis during the Unidirectional Motion of Dimeric Myosin; 3.1. Mechanosensitive detachment of myosin-V from actin; 3.2. Mechanosensitive attachment of myosin-VI to actin 4. Modeling and Simulating Mechanochemical Coupling and Motor Protein Motion4.1. Molecular dynamics simulations; 4.2. Coarse-grained models and dynamics; 4.3. Quantum mechanics for chemical processes; 5. Modeling and Simulations of the Collective Behaviour of Motor Proteins; 5.1. Huxley's 1957 model; 5.2. Huxley and Simmons' 1971 model; 5.3. Diffusional model; References; 5. Nanomotors Propelled by Chemical Reactions Raymond Kapral; 1. Introduction; 2. Propulsion by Phoretic Mechanisms; 3. Microscopic and Mesoscopic Dynamics of Nanomotors; 4. Sphere Dimer Motors; Motor efficiency Motor dynamics in chemically active media |
| Record Nr. | UNINA-9910464000503321 |
| Singapore ; ; Hackensack, NJ, : World Scientific, c2013 | ||
| Materiale a stampa | ||
| Lo trovi qui: Univ. Federico II | ||
| ||
Engineering of chemical complexity [[electronic resource] /] / editors, Alexander S. Mikhailov, Gerhard Ertl
| Engineering of chemical complexity [[electronic resource] /] / editors, Alexander S. Mikhailov, Gerhard Ertl |
| Pubbl/distr/stampa | Singapore ; ; Hackensack, NJ, : World Scientific, c2013 |
| Descrizione fisica | 1 online resource (413 p.) |
| Disciplina |
658.00952
660 |
| Altri autori (Persone) |
MikhailovA. S <1950-> (Alexander S.)
ErtlG (Gerhard) |
| Collana | World Scientific lecture notes in complex systems |
| Soggetto topico |
Chemistry - Mathematics
Chaotic behavior in systems |
| ISBN |
1-283-97146-1
981-4390-46-1 |
| Formato | Materiale a stampa |
| Livello bibliografico | Monografia |
| Lingua di pubblicazione | eng |
| Nota di contenuto |
CONTENTS; Preface; PART I INTRODUCTION; 1. Analysis, Design and Control of Complex Chemical Systems Alexander S. Mikhailov and Gerhard Ertl; 1. Introduction; 2. A Brief Historical Overview; 3. Recent Developments and Open Perspectives; References; PART II SINGLE MOLECULES, NANOSCALE PHENOMENA AND ACTIVE PARTICLES; 2. Imaging and Manipulation of Single Molecules by Scanning Tunneling Microscopy Leonhard Grill; 1. Introduction; 2. Imaging and Spectroscopy of Single Molecules; 2.1. Imaging single molecules; 2.2. Chemical identification by spectroscopy; 2.3. Imaging of diffusion processes
3. Manipulation of Single Molecules3.1. Manipulation without bias voltage; 3.2. Electron-induced manipulation; 3.3. Electric-field induced manipulation; 3.4. Lateral manipulation: Hopping vs rolling; 3.5. Vertical manipulation: Pulling single molecules from a surface; Acknowledgments; References; 3. Self-Organization at the Nanoscale in Far-From- Equilibrium Surface Reactions and Copolymerizations Pierre Gaspard; 1. Introduction; 2. Fundamental Aspects of Nonequilibrium Nanosystems; 2.1. Structure and function of nanosystems; 2.2. Out-of-equilibrium directionality of fluctuating currents 2.3. Thermodynamic origins of dynamical order3. Heterogeneous Catalytic Reactions in High Electric Fields; 3.1. Surface conditions in FEM and FIM; 3.2. Adsorption-desorption kinetics; 3.3. Surface oxides of rhodium; 3.4. The H2-O2/Rh system; 3.4.1. Kinetic equations; 3.4.2. Bistability; 3.4.3. Oscillations; 3.5. Self-organization at the nanoscale; 4. Copolymerization processes; 4.1. Information processing at the molecular scale; 4.2. Thermodynamics of free copolymerization; 4.3. Thermodynamics of copolymerization with a template; 4.4. The case of DNA replication 5. Conclusions and PerspectivesAcknowledgments; References; 4. Single Molecule and Collective Dynamics of Motor Protein Coupled with Mechano-Sensitive Chemical Reaction Mitsuhiro Iwaki, Lorenzo Marcucci, Yuichi Togashi and Toshio Yanagida; 1. What is a Motor Protein?; 2. Measurement of Myosin at the Single Molecule Level; 3. Mechanosensitivity of ATP Hydrolysis during the Unidirectional Motion of Dimeric Myosin; 3.1. Mechanosensitive detachment of myosin-V from actin; 3.2. Mechanosensitive attachment of myosin-VI to actin 4. Modeling and Simulating Mechanochemical Coupling and Motor Protein Motion4.1. Molecular dynamics simulations; 4.2. Coarse-grained models and dynamics; 4.3. Quantum mechanics for chemical processes; 5. Modeling and Simulations of the Collective Behaviour of Motor Proteins; 5.1. Huxley's 1957 model; 5.2. Huxley and Simmons' 1971 model; 5.3. Diffusional model; References; 5. Nanomotors Propelled by Chemical Reactions Raymond Kapral; 1. Introduction; 2. Propulsion by Phoretic Mechanisms; 3. Microscopic and Mesoscopic Dynamics of Nanomotors; 4. Sphere Dimer Motors; Motor efficiency Motor dynamics in chemically active media |
| Record Nr. | UNINA-9910788620403321 |
| Singapore ; ; Hackensack, NJ, : World Scientific, c2013 | ||
| Materiale a stampa | ||
| Lo trovi qui: Univ. Federico II | ||
| ||
Engineering of chemical complexity / / editors, Alexander S. Mikhailov, Gerhard Ertl
| Engineering of chemical complexity / / editors, Alexander S. Mikhailov, Gerhard Ertl |
| Edizione | [1st ed.] |
| Pubbl/distr/stampa | Singapore ; ; Hackensack, NJ, : World Scientific, c2013 |
| Descrizione fisica | 1 online resource (413 p.) |
| Disciplina |
658.00952
660 |
| Altri autori (Persone) |
MikhailovA. S <1950-> (Alexander S.)
ErtlG (Gerhard) |
| Collana | World Scientific lecture notes in complex systems |
| Soggetto topico |
Chemistry - Mathematics
Chaotic behavior in systems |
| ISBN |
1-283-97146-1
981-4390-46-1 |
| Formato | Materiale a stampa |
| Livello bibliografico | Monografia |
| Lingua di pubblicazione | eng |
| Nota di contenuto |
CONTENTS; Preface; PART I INTRODUCTION; 1. Analysis, Design and Control of Complex Chemical Systems Alexander S. Mikhailov and Gerhard Ertl; 1. Introduction; 2. A Brief Historical Overview; 3. Recent Developments and Open Perspectives; References; PART II SINGLE MOLECULES, NANOSCALE PHENOMENA AND ACTIVE PARTICLES; 2. Imaging and Manipulation of Single Molecules by Scanning Tunneling Microscopy Leonhard Grill; 1. Introduction; 2. Imaging and Spectroscopy of Single Molecules; 2.1. Imaging single molecules; 2.2. Chemical identification by spectroscopy; 2.3. Imaging of diffusion processes
3. Manipulation of Single Molecules3.1. Manipulation without bias voltage; 3.2. Electron-induced manipulation; 3.3. Electric-field induced manipulation; 3.4. Lateral manipulation: Hopping vs rolling; 3.5. Vertical manipulation: Pulling single molecules from a surface; Acknowledgments; References; 3. Self-Organization at the Nanoscale in Far-From- Equilibrium Surface Reactions and Copolymerizations Pierre Gaspard; 1. Introduction; 2. Fundamental Aspects of Nonequilibrium Nanosystems; 2.1. Structure and function of nanosystems; 2.2. Out-of-equilibrium directionality of fluctuating currents 2.3. Thermodynamic origins of dynamical order3. Heterogeneous Catalytic Reactions in High Electric Fields; 3.1. Surface conditions in FEM and FIM; 3.2. Adsorption-desorption kinetics; 3.3. Surface oxides of rhodium; 3.4. The H2-O2/Rh system; 3.4.1. Kinetic equations; 3.4.2. Bistability; 3.4.3. Oscillations; 3.5. Self-organization at the nanoscale; 4. Copolymerization processes; 4.1. Information processing at the molecular scale; 4.2. Thermodynamics of free copolymerization; 4.3. Thermodynamics of copolymerization with a template; 4.4. The case of DNA replication 5. Conclusions and PerspectivesAcknowledgments; References; 4. Single Molecule and Collective Dynamics of Motor Protein Coupled with Mechano-Sensitive Chemical Reaction Mitsuhiro Iwaki, Lorenzo Marcucci, Yuichi Togashi and Toshio Yanagida; 1. What is a Motor Protein?; 2. Measurement of Myosin at the Single Molecule Level; 3. Mechanosensitivity of ATP Hydrolysis during the Unidirectional Motion of Dimeric Myosin; 3.1. Mechanosensitive detachment of myosin-V from actin; 3.2. Mechanosensitive attachment of myosin-VI to actin 4. Modeling and Simulating Mechanochemical Coupling and Motor Protein Motion4.1. Molecular dynamics simulations; 4.2. Coarse-grained models and dynamics; 4.3. Quantum mechanics for chemical processes; 5. Modeling and Simulations of the Collective Behaviour of Motor Proteins; 5.1. Huxley's 1957 model; 5.2. Huxley and Simmons' 1971 model; 5.3. Diffusional model; References; 5. Nanomotors Propelled by Chemical Reactions Raymond Kapral; 1. Introduction; 2. Propulsion by Phoretic Mechanisms; 3. Microscopic and Mesoscopic Dynamics of Nanomotors; 4. Sphere Dimer Motors; Motor efficiency Motor dynamics in chemically active media |
| Record Nr. | UNINA-9910812579203321 |
| Singapore ; ; Hackensack, NJ, : World Scientific, c2013 | ||
| Materiale a stampa | ||
| Lo trovi qui: Univ. Federico II | ||
| ||
Preparation of solid catalysts / / edited by G. Ertl, H. Knözinger, J. Weitkamp
| Preparation of solid catalysts / / edited by G. Ertl, H. Knözinger, J. Weitkamp |
| Pubbl/distr/stampa | Weinheim, [Germany] : , : Wiley-VCH, , 1999 |
| Descrizione fisica | 1 online resource (641 p.) |
| Disciplina |
541.3
541.3/95 541.395 |
| Soggetto topico | Metal catalysts |
| Soggetto genere / forma | Electronic books. |
| ISBN |
1-281-76469-8
9786611764692 3-527-61952-6 3-527-62068-0 |
| Formato | Materiale a stampa |
| Livello bibliografico | Monografia |
| Lingua di pubblicazione | eng |
| Nota di contenuto |
Preparation of Solid Catalysts; Contents; 1 Introduction; 2 Developing Industrial Catalysts; 2.1 Properties and Characteristics of Industrial Catalysts; 2.1.1 Activity; 2.1.2 Selectivity; 2.1.3 Stability; 2.1.4 Morphology; 2.1.5 Mechanical Strength; 2.1.6 Thermal Characteristics; 2.1.7 Regenerability; 2.1.8 Reproducibility; 2.1.9 Originality; 2.1.10 Cost; 2.2 The Ideal Catalyst and the Optimum Catalyst; 2.2.1 Catalyst Development; 2.2.2 Devising the First Catalytic Formulas; 2.2.3 Optimization of a Typical Catalytic Formula; 3 Bulk Catalysts and Supports; 3.1 Fused Catalysts
3.1.1 Introduction3.1.2 Concept of Fused Catalysts; 3.1.3 Thermodynamic and Kinetic Considerations; 3.1.4 Sulfuric Acid Catalyst; 3.1.5 Metallic Glasses; 3.1.6 Mesostructure of Fused Catalyst Materials; 3.2 Skeletal Metal Catalysts; 3.2.1 Introduction; 3.2.2 General Aspects; 3.2.3 Skeletal Nickel Catalysts; 3.2.4 Promoted Skeletal Nickel Catalysts; 3.2.5 Skeletal Cobalt Catalysts; 3.2.6 Skeletal Copper Catalysts; 3.2.7 Promoted Skeletal Copper Catalysts; 3.2.8 Skeletal Copper-Zinc Catalysts; 3.3 Metallic Glasses; 3.3.1 Introduction; 3.3.2 Preparation; 3.3.3 Chemical and Structural Properties 3.3.4 Metallic Glasses in Catalysis Research3.3.4.1 Research on Metallic Glasses in As-Quenched State; 3.3.4.2 Metallic Glasses as Precursors to Catalytically Active Materials; 3.3.5 Case Studies: CO Oxidation Catalysts Prepared from Metallic Glasses; 3.3.5.1 Pd/Zr02 Catalysts from Amorphous Pd-Zr Alloys; 3.3.5.2 Promoted Gold-Zirconia Catalysts from Ternary Gold- Containing Glassy Alloys; 3.3.6 Factors Influencing Chemical and Structural Properties of Catalytic Materials Derived from Metallic Glasses; 3.3.6.1 Chemical Composition; 3.3.6.2 Chemical and Structural Homogeneity 3.3.6.3 Thermal Stability and Crystallization Behavior3.3.6.4 Oxidation Behavior; 3.3.6.5 Dissolution of Gases; 3.3.6.6 Segregation Phenomena; 3.3.7 Conclusions and Outlook; 3.4 Precipitation and Coprecipitation; 3.4.1 Introduction; 3.4.2 General Principles Governing Precipitation from Solutions; 3.4.3 Influencing the Properties of the Final Product; 3.4.4 Prototypical Examples of Precipitated Catalysts and Supports; 3.5 Sol-Gel Process; 3.5.1 Introduction; 3.5.2 Important Parameters in Sol-Gel Preparation; 3.5.3 Advantages of Sol-Gel Preparation; 3.5.4 Catalytic Membranes 3.5.5 Other Sol-Gel Materials3.5.6 Summary; 3.6 Flame Hydrolysis; 3.6.1 Manufacture; 3.6.2 Physicochemical Properties of Fumed Oxides; 3.6.3 Preparation of Formed Supports; 3.7 Solid-state Reactions; 3.7.1 Why Solid-state Reactions?; 3.7.2 Description of Preparative Methods; 3.7.3 Conclusions and Prospects; 3.8 High-Surface Transition Metal Carbides and Nitrides; 3.8.1 General Properties of Transition Metal Carbides and Nitrides; 3.8.2 Thermodynamic Considerations in the Preparation of Carbides and Nitrides; 3.8.3 Survey of Preparative Methods; 3.9 Carbons; 3.9.1 Introduction 3.9.2 Structural Chemistry of Carbon |
| Record Nr. | UNINA-9910144133003321 |
| Weinheim, [Germany] : , : Wiley-VCH, , 1999 | ||
| Materiale a stampa | ||
| Lo trovi qui: Univ. Federico II | ||
| ||
Preparation of solid catalysts / / edited by G. Ertl, H. Knözinger, J. Weitkamp
| Preparation of solid catalysts / / edited by G. Ertl, H. Knözinger, J. Weitkamp |
| Pubbl/distr/stampa | Weinheim, [Germany] : , : Wiley-VCH, , 1999 |
| Descrizione fisica | 1 online resource (641 p.) |
| Disciplina |
541.3
541.3/95 541.395 |
| Soggetto topico | Metal catalysts |
| ISBN |
1-281-76469-8
9786611764692 3-527-61952-6 3-527-62068-0 |
| Formato | Materiale a stampa |
| Livello bibliografico | Monografia |
| Lingua di pubblicazione | eng |
| Nota di contenuto |
Preparation of Solid Catalysts; Contents; 1 Introduction; 2 Developing Industrial Catalysts; 2.1 Properties and Characteristics of Industrial Catalysts; 2.1.1 Activity; 2.1.2 Selectivity; 2.1.3 Stability; 2.1.4 Morphology; 2.1.5 Mechanical Strength; 2.1.6 Thermal Characteristics; 2.1.7 Regenerability; 2.1.8 Reproducibility; 2.1.9 Originality; 2.1.10 Cost; 2.2 The Ideal Catalyst and the Optimum Catalyst; 2.2.1 Catalyst Development; 2.2.2 Devising the First Catalytic Formulas; 2.2.3 Optimization of a Typical Catalytic Formula; 3 Bulk Catalysts and Supports; 3.1 Fused Catalysts
3.1.1 Introduction3.1.2 Concept of Fused Catalysts; 3.1.3 Thermodynamic and Kinetic Considerations; 3.1.4 Sulfuric Acid Catalyst; 3.1.5 Metallic Glasses; 3.1.6 Mesostructure of Fused Catalyst Materials; 3.2 Skeletal Metal Catalysts; 3.2.1 Introduction; 3.2.2 General Aspects; 3.2.3 Skeletal Nickel Catalysts; 3.2.4 Promoted Skeletal Nickel Catalysts; 3.2.5 Skeletal Cobalt Catalysts; 3.2.6 Skeletal Copper Catalysts; 3.2.7 Promoted Skeletal Copper Catalysts; 3.2.8 Skeletal Copper-Zinc Catalysts; 3.3 Metallic Glasses; 3.3.1 Introduction; 3.3.2 Preparation; 3.3.3 Chemical and Structural Properties 3.3.4 Metallic Glasses in Catalysis Research3.3.4.1 Research on Metallic Glasses in As-Quenched State; 3.3.4.2 Metallic Glasses as Precursors to Catalytically Active Materials; 3.3.5 Case Studies: CO Oxidation Catalysts Prepared from Metallic Glasses; 3.3.5.1 Pd/Zr02 Catalysts from Amorphous Pd-Zr Alloys; 3.3.5.2 Promoted Gold-Zirconia Catalysts from Ternary Gold- Containing Glassy Alloys; 3.3.6 Factors Influencing Chemical and Structural Properties of Catalytic Materials Derived from Metallic Glasses; 3.3.6.1 Chemical Composition; 3.3.6.2 Chemical and Structural Homogeneity 3.3.6.3 Thermal Stability and Crystallization Behavior3.3.6.4 Oxidation Behavior; 3.3.6.5 Dissolution of Gases; 3.3.6.6 Segregation Phenomena; 3.3.7 Conclusions and Outlook; 3.4 Precipitation and Coprecipitation; 3.4.1 Introduction; 3.4.2 General Principles Governing Precipitation from Solutions; 3.4.3 Influencing the Properties of the Final Product; 3.4.4 Prototypical Examples of Precipitated Catalysts and Supports; 3.5 Sol-Gel Process; 3.5.1 Introduction; 3.5.2 Important Parameters in Sol-Gel Preparation; 3.5.3 Advantages of Sol-Gel Preparation; 3.5.4 Catalytic Membranes 3.5.5 Other Sol-Gel Materials3.5.6 Summary; 3.6 Flame Hydrolysis; 3.6.1 Manufacture; 3.6.2 Physicochemical Properties of Fumed Oxides; 3.6.3 Preparation of Formed Supports; 3.7 Solid-state Reactions; 3.7.1 Why Solid-state Reactions?; 3.7.2 Description of Preparative Methods; 3.7.3 Conclusions and Prospects; 3.8 High-Surface Transition Metal Carbides and Nitrides; 3.8.1 General Properties of Transition Metal Carbides and Nitrides; 3.8.2 Thermodynamic Considerations in the Preparation of Carbides and Nitrides; 3.8.3 Survey of Preparative Methods; 3.9 Carbons; 3.9.1 Introduction 3.9.2 Structural Chemistry of Carbon |
| Record Nr. | UNINA-9910830095203321 |
| Weinheim, [Germany] : , : Wiley-VCH, , 1999 | ||
| Materiale a stampa | ||
| Lo trovi qui: Univ. Federico II | ||
| ||