LEADER 05334oam 2200541 450 001 9910808017203321 005 20190911112729.0 010 $a981-4518-34-4 035 $a(OCoLC)897427178 035 $a(MiFhGG)GVRL8RHH 035 $a(EXLCZ)992550000001191470 100 $a20141111h20142014 uy 0 101 0 $aeng 135 $aurun|---uuuua 181 $ctxt 182 $cc 183 $acr 200 00$aAdvances in multi-photon processes and spectroscopy$hVolume 21 /$fedited by S.H. Lin, National Chiao-Tung University, Taiwan, Institute of Atomic and Molecular Sciences, Taiwan and Arizona State University, USA, A.A. Villaeys, Institute de Physique et Chimie des Materiaux de Strasbourg, France, Y. Fujimura, Tohoku University, Japan 210 1$aNew Jersey :$cWorld Scientific,$d[2014] 210 4$d?2014 215 $a1 online resource (xii, 244 pages) $cillustrations (some color) 225 1 $aAdvances in Multi-Photon Processes and Spectroscopy 300 $aDescription based upon print version of record. 311 $a981-4518-33-6 311 $a1-306-39642-5 320 $aIncludes bibliographical references. 327 $aPreface; CONTENTS; 1. Vibrational and Electronic Wavepackets Driven by Strong Field Multiphoton Ionization; 1.1 Introduction; 1.2 Theoretical Concepts; 1.2.1 The time-independent Schro?dinger equation and its implications on dynamics; 1.2.2 Spin-orbit coupling and diabatic vs. adiabatic states; 1.2.3 Nuclear time-dependent Schro?dinger equation; 1.2.3.1 Second-order differentiator; 1.2.3.2 Split-operator method; 1.2.4 Stark shifts; 1.2.5 Multi- vs. single-photon transitions; 1.2.6 Laser-dressed states; 1.2.7 Photon locking; 1.2.8 Hole burning; 1.2.9 Strong-field ionization 327 $a1.3 Computational and experimental details 1.4 Vibrational Wavepackets Created by Multiphoton Ionization; 1.4.1 Phase-dependent dissociation; 1.4.1.1 Photon locking; 1.4.1.2 Hole burning; 1.4.2 Ionization to different ionic states; 1.4.2.1 Preparing electronic wavepackets via SFI; 1.4.2.2 VMI measurements to identify dissociation pathways following SFI; 1.5 Conclusion and Outlook; References; 2. Orientation-Selective Molecular Tunneling Ionization by Phase-Controlled Laser Fields; 1 Introduction; 2 Photoionization Induced by Intense Laser Fields; 2.1 MPI in standard perturbation theory 327 $a2.2 Keldysh theory: From MPI to TI2.3 Characteristics of TI; 2.4 Molecular TI; 3 Directionally Asymmetric TI Induced by Phase-controlled Laser Fields; 3.1 Phase-controlled laser fields; 3.2 Directionally asymmetric TI (atoms); 3.3 Directionally asymmetric TI (molecules); 4 Experimental; 5 Results and Discussion; 5.1 Diatomic molecule: CO; 5.1.1 Photo fragment detection; 5.1.2 Photoelectron detection; 5.2 Other molecules; 5.2.1 Nonpolar molecule with asymmetric structure: Br(CH2)2 Cl; 5.2.2 Large molecule: C6H13I; 5.2.3 Systematically changing molecular system: CH3X(X=F,Cl,Br, I) 327 $a5.2.4 OCS molecule investigated by nanosecond ? + 2? laser fields 6 Summary; Acknowledgments; References; 3. Reaction and Ionization of Polyatomic Molecules Induced by Intense Laser Pulses; 1.1 Introduction; 1.2 Ionization Rate of Molecules in Intense Laser Fields; 1.2.1 Theoretical approaches for ionization rates of molecules in intense laser fields; 1.2.2 Experimental measurements of ionization rates of molecules and comparations with theory; 1.3 Fragmentation of Molecules in Intense Laser Fields 327 $a1.3.1 Ionization-dissociation of molecules in intense laser fields and statistical theoretical description 1.3.2 Effects of cation absorption on molecular dissociation; 1.4 Dissociative Ionization and Coulombic Explosion of Molecules in Intense Laser Fields; 1.4.1 Dissociative ionization of formic acid molecules; 1.4.2 Coulombic explosion of CH3I; 1.5 Summary and Perspectives; Acknowledgments; References; 4. Ultrafast Internal Conversion of Pyrazine Via Conical Intersection; 1.1 Introduction; 1.2 Pyrazine: Ultrafast S2(1B2u, ??*) - S1(1B3u, n?*) Internal Conversion Via Conical Intersection 327 $a1.3 Sub-20 fs Deep UV Laser for TRPEI of Pyrazine 330 $aThis volume presents recent progress and perspectives in multi-photon processes and spectroscopy of atoms, ions, molecules and solids. The subjects in the series cover the experimental and theoretical investigations in the interdisciplinary research fields of natural science including chemistry, physics, bioscience and material science. This volume is the latest volume in a series that is a pioneer in compiling review articles of nonlinear interactions of photons and matter. It has made an essential contribution to the development and promotion of the related research fields. In view of the ra 410 0$aAdvances in Multi-Photon Processes and Spectroscopy 606 $aMultiphoton processes 606 $aMolecular spectroscopy 615 0$aMultiphoton processes. 615 0$aMolecular spectroscopy. 676 $a257 702 $aLin$b S. H$g(Sheng Hsien),$f1937- 702 $aVillaeys$b A. A. 702 $aFujimura$b Y$g(Yuichi), 801 0$bMiFhGG 801 1$bMiFhGG 906 $aBOOK 912 $a9910808017203321 996 $aAdvances in multi-photon processes and spectroscopy$94021858 997 $aUNINA