LEADER 03540nam 22007335 450 001 9910484164303321 005 20251202165448.0 010 $a3-030-70940-X 024 7 $a10.1007/978-3-030-70940-2 035 $a(CKB)4100000011930316 035 $a(DE-He213)978-3-030-70940-2 035 $a(MiAaPQ)EBC6627522 035 $a(Au-PeEL)EBL6627522 035 $a(OCoLC)1252424823 035 $a(PPN)255883056 035 $a(EXLCZ)994100000011930316 100 $a20210518d2021 u| 0 101 0 $aeng 135 $aurnn|008mamaa 181 $ctxt$2rdacontent 182 $cc$2rdamedia 183 $acr$2rdacarrier 200 10$aExciton Dynamics in Lead Halide Perovskite Nanocrystals $eRecombination, Dephasing and Diffusion /$fby Bernhard Johann Bohn 205 $a1st ed. 2021. 210 1$aCham :$cSpringer International Publishing :$cImprint: Springer,$d2021. 215 $a1 online resource (XXII, 152 p. 62 illus., 58 illus. in color.) 225 1 $aSpringer Theses, Recognizing Outstanding Ph.D. Research,$x2190-5061 311 08$a3-030-70939-6 327 $aIntroduction -- Fundamentals -- Materials and Methods -- Recombination -- Dephasing -- Diffusion. 330 $aLess than a decade ago, lead halide perovskite semiconductors caused a sensation: Solar cells exhibiting astonishingly high levels of efficiency. Recently, it became possible to synthesize nanocrystals of this material as well. Interestingly; simply by controlling the size and shape of these crystals, new aspects of this material literally came to light. These nanocrystals have proven to be interesting candidates for light emission. In this thesis, the recombination, dephasing and diffusion of excitons in perovskite nanocrystals is investigated using time-resolved spectroscopy. All these dynamic processes have a direct impact on the light-emitting device performance from a technology point of view. However, most importantly, the insights gained from the measurements allowed the author to modify the nanocrystals such that they emitted with an unprecedented quantum yield in the blue spectral range, resulting in the successful implementation of this material as the activelayer in an LED. This represents a technological breakthrough, because efficient perovskite light emitters in this wavelength range did not exist before. 410 0$aSpringer Theses, Recognizing Outstanding Ph.D. Research,$x2190-5061 606 $aNanoscience 606 $aPhotovoltaic power generation 606 $aOptical spectroscopy 606 $aNanoparticles 606 $aElectronics$xMaterials 606 $aOptical materials 606 $aNanophysics 606 $aPhotovoltaics 606 $aOptical Spectroscopy 606 $aNanoparticles 606 $aElectronic Materials 606 $aOptical Materials 615 0$aNanoscience. 615 0$aPhotovoltaic power generation. 615 0$aOptical spectroscopy. 615 0$aNanoparticles. 615 0$aElectronics$xMaterials. 615 0$aOptical materials. 615 14$aNanophysics. 615 24$aPhotovoltaics. 615 24$aOptical Spectroscopy. 615 24$aNanoparticles. 615 24$aElectronic Materials. 615 24$aOptical Materials. 676 $a621.38152 700 $aBohn$b Bernhard Johann$0946975 801 0$bMiAaPQ 801 1$bMiAaPQ 801 2$bMiAaPQ 906 $aBOOK 912 $a9910484164303321 996 $aExciton Dynamics in Lead Halide Perovskite Nanocrystals$92139505 997 $aUNINA