LEADER 05858nam 2200733 450 001 9910453659703321 005 20200520144314.0 010 $a981-4518-34-4 035 $a(CKB)2550000001191470 035 $a(EBL)1611967 035 $a(SSID)ssj0001152167 035 $a(PQKBManifestationID)11660341 035 $a(PQKBTitleCode)TC0001152167 035 $a(PQKBWorkID)11147911 035 $a(PQKB)10953042 035 $a(MiAaPQ)EBC1611967 035 $a(WSP)00008851 035 $a(Au-PeEL)EBL1611967 035 $a(CaPaEBR)ebr10832722 035 $a(OCoLC)870245931 035 $a(EXLCZ)992550000001191470 100 $a20140205h20142014 uy| 0 101 0 $aeng 135 $aurcnu|||||||| 181 $ctxt 182 $cc 183 $acr 200 00$aAdvances in multi-photon processes and spectroscopy$hVolume 21 /$fedited by S.H. Lin, National Chiao-Tung University, Taiwan, Institute of Atomic and Molecular Sciences, Taiwan and Arizona State University, USA, A.A. Villaeys, Institute de Physique et Chimie des Mate?riaux de Strasbourg, France, Y. Fujimura, Tohoku University, Japan 210 1$aNew Jersey :$cWorld Scientific Publishing Compan,$d[2014] 210 4$dİ2014 215 $a1 online resource (257 p.) 225 1 $aAdvances in Multi-Photon Processes and Spectroscopy 300 $aDescription based upon print version of record. 311 $a981-4518-33-6 311 $a1-306-39642-5 320 $aIncludes bibliographical references. 327 $aPreface; CONTENTS; 1. Vibrational and Electronic Wavepackets Driven by Strong Field Multiphoton Ionization; 1.1 Introduction; 1.2 Theoretical Concepts; 1.2.1 The time-independent Schro?dinger equation and its implications on dynamics; 1.2.2 Spin-orbit coupling and diabatic vs. adiabatic states; 1.2.3 Nuclear time-dependent Schro?dinger equation; 1.2.3.1 Second-order differentiator; 1.2.3.2 Split-operator method; 1.2.4 Stark shifts; 1.2.5 Multi- vs. single-photon transitions; 1.2.6 Laser-dressed states; 1.2.7 Photon locking; 1.2.8 Hole burning; 1.2.9 Strong-field ionization 327 $a1.3 Computational and experimental details 1.4 Vibrational Wavepackets Created by Multiphoton Ionization; 1.4.1 Phase-dependent dissociation; 1.4.1.1 Photon locking; 1.4.1.2 Hole burning; 1.4.2 Ionization to different ionic states; 1.4.2.1 Preparing electronic wavepackets via SFI; 1.4.2.2 VMI measurements to identify dissociation pathways following SFI; 1.5 Conclusion and Outlook; References; 2. Orientation-Selective Molecular Tunneling Ionization by Phase-Controlled Laser Fields; 1 Introduction; 2 Photoionization Induced by Intense Laser Fields; 2.1 MPI in standard perturbation theory 327 $a2.2 Keldysh theory: From MPI to TI2.3 Characteristics of TI; 2.4 Molecular TI; 3 Directionally Asymmetric TI Induced by Phase-controlled Laser Fields; 3.1 Phase-controlled laser fields; 3.2 Directionally asymmetric TI (atoms); 3.3 Directionally asymmetric TI (molecules); 4 Experimental; 5 Results and Discussion; 5.1 Diatomic molecule: CO; 5.1.1 Photo fragment detection; 5.1.2 Photoelectron detection; 5.2 Other molecules; 5.2.1 Nonpolar molecule with asymmetric structure: Br(CH2)2 Cl; 5.2.2 Large molecule: C6H13I; 5.2.3 Systematically changing molecular system: CH3X(X=F,Cl,Br, I) 327 $a5.2.4 OCS molecule investigated by nanosecond ? + 2? laser fields 6 Summary; Acknowledgments; References; 3. Reaction and Ionization of Polyatomic Molecules Induced by Intense Laser Pulses; 1.1 Introduction; 1.2 Ionization Rate of Molecules in Intense Laser Fields; 1.2.1 Theoretical approaches for ionization rates of molecules in intense laser fields; 1.2.2 Experimental measurements of ionization rates of molecules and comparations with theory; 1.3 Fragmentation of Molecules in Intense Laser Fields 327 $a1.3.1 Ionization-dissociation of molecules in intense laser fields and statistical theoretical description 1.3.2 Effects of cation absorption on molecular dissociation; 1.4 Dissociative Ionization and Coulombic Explosion of Molecules in Intense Laser Fields; 1.4.1 Dissociative ionization of formic acid molecules; 1.4.2 Coulombic explosion of CH3I; 1.5 Summary and Perspectives; Acknowledgments; References; 4. Ultrafast Internal Conversion of Pyrazine Via Conical Intersection; 1.1 Introduction; 1.2 Pyrazine: Ultrafast S2(1B2u, ??*) - S1(1B3u, n?*) Internal Conversion Via Conical Intersection 327 $a1.3 Sub-20 fs Deep UV Laser for TRPEI of Pyrazine 330 $aThis volume presents recent progress and perspectives in multi-photon processes and spectroscopy of atoms, ions, molecules and solids. The subjects in the series cover the experimental and theoretical investigations in the interdisciplinary research fields of natural science including chemistry, physics, bioscience and material science. This volume is the latest volume in a series that is a pioneer in compiling review articles of nonlinear interactions of photons and matter. It has made an essential contribution to the development and promotion of the related research fields. In view of the ra 410 0$aAdvances in Multi-Photon Processes and Spectroscopy 606 $aMultiphoton processes 606 $aSpectrum analysis 606 $aLaser spectroscopy 606 $aMolecular spectra 608 $aElectronic books. 615 0$aMultiphoton processes. 615 0$aSpectrum analysis. 615 0$aLaser spectroscopy. 615 0$aMolecular spectra. 676 $a257 701 $aLin$b S. H$0898770 701 $aVillaeys$b A. A$0898771 701 $aFujimura$b Y$0321391 801 0$bMiAaPQ 801 1$bMiAaPQ 801 2$bMiAaPQ 906 $aBOOK 912 $a9910453659703321 996 $aAdvances in multi-photon processes and spectroscopy$92007995 997 $aUNINA