LEADER 01558cam0-22004211i-450- 001 990004331640403321 005 20140714142306.0 010 $a88-311-9136-5 035 $a000433164 035 $aFED01000433164 035 $a(Aleph)000433164FED01 035 $a000433164 100 $a19990604d1992----km-y0itay50------ba 101 2 $alat$aita 102 $aIT 105 $af---e---001yy 200 1 $a<>dottrina cristiana$etesto latino dell'edizione mauriana confrontato con il corpus scriptorum ecclesiasticorum latinorum$fSant'Agostino$gintroduzione generale di Mario Naldini, Luigi Alici, Antonio Quacquarelli, Prospero Grech; traduzione di Vincenzo Tarulli ; indici di Franco Monteverde 210 $aRoma$cCitta' Nuova editrice$dc1992 215 $aXCV, 320 p., [4] c.ditav.$d25 cm 225 1 $aNuova biblioteca agostiniana. Opere di Sant'Agostino. Parte I$eOpere esegetiche$v8 500 10$aDe doctrina christiana$min latino e italiano$921768 676 $a189$v11 rid.$zita 700 1$aAugustinus,$bAurelius$f<354-430>$0152280 702 1$aAlici,$bLuigi$f<1959- > 702 1$aGrech,$bProspero 702 1$aMonteverde,$bFranco 702 1$aNaldini,$bMario 702 1$aQuacquarelli,$bAntonio$f<1918-2001> 702 1$aTarulli,$bVincenzo 801 0$aIT$bUNINA$gRICA$2UNIMARC 901 $aBK 912 $a990004331640403321 952 $a870.08CH.NBA(8)$bBibl.12972$fFLFBC 952 $aXI CL S 12 (9)$b481$fDFD 959 $aFLFBC 959 $aDFD 996 $aDe doctrina christiana$921768 997 $aUNINA LEADER 03803nam 22006495 450 001 9910427687703321 005 20251202165837.0 010 $a3-030-54851-1 024 7 $a10.1007/978-3-030-54851-3 035 $a(CKB)4100000011435701 035 $a(DE-He213)978-3-030-54851-3 035 $a(MiAaPQ)EBC6348293 035 $a(PPN)250221527 035 $a(MiAaPQ)EBC29092957 035 $a(EXLCZ)994100000011435701 100 $a20200910d2020 u| 0 101 0 $aeng 135 $aurnn|008mamaa 181 $ctxt$2rdacontent 182 $cc$2rdamedia 183 $acr$2rdacarrier 200 10$aChemistry in Action: Making Molecular Movies with Ultrafast Electron Diffraction and Data Science /$fby Lai Chung Liu 205 $a1st ed. 2020. 210 1$aCham :$cSpringer International Publishing :$cImprint: Springer,$d2020. 215 $a1 online resource (XX, 239 p. 110 illus., 106 illus. in color.) 225 1 $aSpringer Theses, Recognizing Outstanding Ph.D. Research,$x2190-5061 311 08$a3-030-54850-3 327 $aChapter1: Introduction -- Chapter2: Methods: Experimental Techniques and Data Science -- Chapter3: Ultrafast Structural Dynamics of (EDO-TTF)2X -- Chapter4: Photocyclization Dynamics of Diarylethene -- Chapter5: Photoinduced Spin Crossover in Iron(II) Systems -- Chapter6: Future Work -- Chapter7: Conclusion. 330 $aThe thesis provides the necessary experimental and analytical tools to unambiguously observe the atomically resolved chemical reactions. A great challenge of modern science has been to directly observe atomic motions during structural transitions, and while this was first achieved through a major advance in electron source brightness, the information content was still limited and new methods for image reconstruction using femtosecond electron diffraction methods were needed. One particular challenge lay in reconciling the innumerable possible nuclear configurations with the observation of chemical reaction mechanisms that reproducibly give the same kind of chemistry for large classes of molecules. The author shows that there is a simple solution that occurs during barrier crossing in which the highly anharmonic potential at that point in nuclear rearrangements couples high- and low-frequency vibrational modes to give highly localized nuclear motions, reducing hundreds of potentialdegrees of freedom to just a few key modes. Specific examples are given in this thesis, including two photoinduced phase transitions in an organic system, a ring closure reaction, and two direct observations of nuclear reorganization driven by spin transitions. The emerging field of structural dynamics promises to change the way we think about the physics of chemistry and this thesis provides tools to make it happen. 410 0$aSpringer Theses, Recognizing Outstanding Ph.D. Research,$x2190-5061 606 $aMolecular spectroscopy 606 $aMolecular dynamics 606 $aElectrons$xDiffraction 606 $aInstrumental analysis 606 $aCrystallography 606 $aMolecular Spectroscopy 606 $aMolecular Dynamics 606 $aDiffraction 606 $aCrystallography and Scattering Methods 615 0$aMolecular spectroscopy. 615 0$aMolecular dynamics. 615 0$aElectrons$xDiffraction. 615 0$aInstrumental analysis. 615 0$aCrystallography. 615 14$aMolecular Spectroscopy. 615 24$aMolecular Dynamics. 615 24$aDiffraction. 615 24$aCrystallography and Scattering Methods. 676 $a541.223 700 $aLiu$b Lai Chung$0841964 801 0$bMiAaPQ 801 1$bMiAaPQ 801 2$bMiAaPQ 906 $aBOOK 912 $a9910427687703321 996 $aChemistry in action$92057019 997 $aUNINA